Wang Jiaqi, Xu Jinkai, Chen Guangjun, Lian Zhongxu, Yu Huadong
Ministry of Education Key Laboratory for Cross-Scale Micro and Nano Manufacturing, Changchun University of Science and Technology, Changchun 130022, China.
ACS Omega. 2020 Dec 17;6(1):77-84. doi: 10.1021/acsomega.0c03369. eCollection 2021 Jan 12.
Design and fabrication of smart materials with reversible wettability for oil-water separation have attracted worldwide attention due to the increasingly serious water pollution problem. In this study, a rough oxide coating with micro/nanoscale structures is developed on the 304 stainless steel mesh (SSM) by laser ablation. The smart surface with ethanol immersion and natural drying treatments shows the wetting conversion between underwater superoleophobicity and superhydrophobicity. Based on the wettability transition behavior, both light and heavy oil-water mixtures can be separated with the high separation efficiency. Moreover, after being exposed to various corrosive solutions and high temperatures, the smart surface still shows prominent environmental stability. Switchable surface with excellent properties should be an optimal choice to solve the environmental conditions that need to be addressed urgently.
由于水污染问题日益严重,具有可逆润湿性的智能材料用于油水分离的设计与制备已引起全球关注。在本研究中,通过激光烧蚀在304不锈钢网(SSM)上制备了具有微/纳米级结构的粗糙氧化物涂层。经过乙醇浸泡和自然干燥处理的智能表面展现出水下超疏油性和超疏水性之间的润湿转变。基于这种润湿性转变行为,轻质和重质油水混合物均可实现高效分离。此外,在暴露于各种腐蚀性溶液和高温后,该智能表面仍表现出出色的环境稳定性。具有优异性能的可切换表面应是解决迫切需要应对的环境条件的最佳选择。