Materials Science Division, Argonne National Laboratory, Lemont, IL 60439, USA.
Advanced Photon Source, Argonne National Laboratory, Lemont, IL 60439, USA.
Science. 2021 Feb 12;371(6530):716-721. doi: 10.1126/science.aba5511. Epub 2021 Jan 21.
The distinctive electronic structure found at interfaces between materials can allow unconventional quantum states to emerge. Here we report on the discovery of superconductivity in electron gases formed at interfaces between (111)-oriented KTaO and insulating overlayers of either EuO or LaAlO The superconducting transition temperature, as high as 2.2 kelvin, is about one order of magnitude higher than that of the LaAlO/SrTiO system. Notably, similar electron gases at KTaO (001) interfaces remain normal down to 25 millikelvin. The critical field and current-voltage measurements indicate that the superconductivity is two-dimensional. In EuO/KTaO (111) samples, a spontaneous in-plane transport anisotropy is observed before the onset of superconductivity, suggesting the emergence of a distinct "stripe"-like phase, which is also revealed near the critical field.
在材料界面处发现的独特电子结构可以允许非常规量子态出现。在这里,我们报告了在(111)取向的 KTaO 和 EuO 或 LaAlO 绝缘覆盖层之间形成的电子气中发现超导性的情况。超导转变温度高达 2.2 开尔文,比 LaAlO/SrTiO 系统高出约一个数量级。值得注意的是,在 KTaO(001)界面处的类似电子气在 25 毫开尔文以下仍保持正常。临界场和电流-电压测量表明超导性是二维的。在 EuO/KTaO(111)样品中,在超导开始之前观察到自发的面内输运各向异性,表明出现了一种独特的“条纹”样相,在临界场附近也可以发现。