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美国陆地区域背景与天然放射性物质整治标准之间的关系。

Relationship Between Terrestrial Background and Remedial Criteria for Naturally Occurring Radioactive Material in the United States.

机构信息

SHB Inc., 7505 S. Xanthia Place, Centennial, CO 80112.

出版信息

Health Phys. 2021 Apr 1;120(4):472-482. doi: 10.1097/HP.0000000000001389.

Abstract

In the United States (US), Federal and State agencies have established radiological public exposure limits and remedial action ("clean up") criteria for naturally occurring radionuclides (NORM-primarily for uranium and thorium series radionuclides). Often, these criteria are intended to control human exposure to what is referred to in the US as technologically enhanced naturally occurring radioactive material (TENORM). This can be any naturally occurring radioactive material for which the potential for human exposure has been enhanced due to anthropogenic (human activities), e.g., removal from its "place in nature," and/or processed in some way resulting in concentration. In some cases, the values of these regulatory criteria can be similar to or even less than those levels of exposure and those concentrations of NORM that exists in nature independent of any previous human activity. The potential variability of NORM radionuclides in the soil and rocks can be significant, even over relatively short distances or depths due to factors such as geology, hydrology, and geochemistry. Given this, it is important to recognize that defining "the radiation background" for purposes of establishing and/or comparing remedial action criteria and/or exposure limits requires recognition of the specificity at the location(s) of interest, not in other geological and/or mineralogical regimes several miles away. The purpose of this paper is to demonstrate this variability for comparison to exposure levels and concentrations being defined in the US as levels above which require regulatory control and / or above which are being defined as an "unacceptable risk." The primary background exposure component of specific interest here is the annual dose contribution from terrestrial radiation exposure, i.e., from uranium and thorium series radionuclides in the ground, excluding radon inhalation. The exposure sources being controlled by some US regulatory limits are primarily associated with the primordial radionuclides in soil. The average annual terrestrial component of background can vary by upwards of a few tenths of a mSv across the US that can be several times higher than the applicable exposure limits. This can result in "unacceptable risk" or "remedial action" concentration criteria statistically equivalent to or less than the background concentrations of these same primordial nuclides. The statistical and analytical uncertainties of distinguishing naturally occurring radionuclides (i.e., NORM) from those resulting from anthropogenic (human caused) activities (i.e., TENORM) can be quite challenging and in some cases may be technically impossible. Consideration must be given to the relationship of the amount of actual total risk avoidance achieved if any, relative to the traditional health and safety risks of construction and associated construction and waste management costs for remedial activities, so that a practical and scientifically based approach for development of these criteria can be achieved.

摘要

在美国,联邦和州机构已经制定了放射性公众暴露限值和补救行动(“清理”)标准,用于天然放射性核素(主要是铀和钍系列放射性核素)。这些标准通常旨在控制人类接触美国所谓的技术增强型天然放射性物质(TENORM)。这可以是任何天然放射性物质,由于人为(人类活动)而增加了人类接触的可能性,例如,将其从“自然位置”中移除,以及/或以某种方式进行处理,导致浓度增加。在某些情况下,这些监管标准的值可能与自然存在的、与任何先前人类活动无关的暴露水平和 TENORM 浓度相似,甚至更低。由于地质、水文和地球化学等因素,土壤和岩石中 NORM 放射性核素的潜在变异性可能很大,即使在相对较短的距离或深度内也是如此。考虑到这一点,重要的是要认识到,为了制定和/或比较补救行动标准和/或暴露限值,为目的定义“辐射背景”需要认识到在感兴趣的地点(多个)的特殊性,而不是在几英里外的其他地质和/或矿物学区域。本文的目的是为了展示这种变异性,以便与美国定义的需要监管控制的水平和/或被定义为“不可接受风险”的水平进行比较。这里特别感兴趣的主要背景暴露成分是来自陆地辐射暴露的年度剂量贡献,即来自地面上的铀和钍系列放射性核素,不包括氡吸入。一些美国监管限值控制的暴露源主要与土壤中的原始放射性核素有关。在美国,背景的陆地成分平均每年可变化几十分之一毫西弗(mSv),这可能是适用的暴露限值的几倍。这可能导致“不可接受的风险”或“补救行动”浓度标准与这些原始核素的背景浓度相同或更低。从人为(人类引起的)活动(即 TENORM)中区分天然放射性核素(即 NORM)的统计和分析不确定性可能相当具有挑战性,在某些情况下可能在技术上是不可能的。必须考虑到如果有任何实际的总风险避免量,相对于补救活动的施工和相关施工及废物管理成本的传统健康和安全风险的关系,以便能够为制定这些标准制定一种实际和基于科学的方法。

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