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霜的静电跳跃

Electrostatic Jumping of Frost.

作者信息

Mukherjee Ranit, Ahmadi S Farzad, Zhang Hongwei, Qiao Rui, Boreyko Jonathan B

机构信息

Department of Biomedical Engineering and Mechanics, Virginia Tech, Blacksburg, Virginia 24061, United States.

Department of Mechanical Engineering, Virginia Tech, Blacksburg, Virginia 24061, United States.

出版信息

ACS Nano. 2021 Mar 23;15(3):4669-4677. doi: 10.1021/acsnano.0c09153. Epub 2021 Feb 24.

Abstract

The electrification of ice has been a subject of research since 1940, mostly in the context of charge generation in thunderstorms. This generation of electric charge is spontaneous, distinct from applying an external electric field to affect the diffusive growth of ice crystals. Here, we exploit the spontaneous electrification of ice to reveal a surprising phenomenon of jumping frost dendrites. We use side-view high-speed imaging to experimentally observe frost dendrites breaking off from mother dendrites and/or the substrate to jump out-of-plane toward an opposing polar liquid. Analytical and numerical models are then developed to estimate the attractive force between the frost dendrites and liquid, in good agreement with the experimental results. These models estimate the extent of charge separation within a growing sheet of frost, which is caused by mismatches in the mobilities of the charge carriers in ice. Our findings show that the unexpected jumping frost event can serve as a model system for resolving long-standing questions in atmospheric physics regarding charge separation in ice, while also having potential as a deicing construct.

摘要

自1940年以来,冰的起电现象一直是研究的课题,主要是在雷暴中电荷产生的背景下。这种电荷的产生是自发的,不同于施加外部电场来影响冰晶的扩散生长。在这里,我们利用冰的自发起电现象揭示了跳变霜枝晶这一惊人现象。我们使用侧视高速成像实验观察霜枝晶从母枝晶和/或基底上脱落,并向相反极性的液体进行面外跳跃。然后建立分析模型和数值模型来估算霜枝晶与液体之间的吸引力,与实验结果吻合良好。这些模型估算了生长的霜层内电荷分离的程度,这是由冰中电荷载流子迁移率的不匹配引起的。我们的研究结果表明,这一意外的跳变霜事件可作为一个模型系统,用于解决大气物理学中关于冰中电荷分离的长期问题,同时也具有作为除冰结构的潜力。

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