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季风期间,北印度恒河平原溶解态氮和有机碳的浓度、来源和湿沉降。

Concentration, sources and wet deposition of dissolved nitrogen and organic carbon in the Northern Indo-Gangetic Plain during monsoon.

机构信息

Earth System Science Programme and Graduate Division of Earth and Atmospheric Sciences, The Chinese University of Hong Kong, Hong Kong, China; Himalayan Environment Research Institute (HERI), Kathmandu, Nepal; Kathmandu Center for Research and Education (KCRE), Kathmandu, Nepal.

State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou 730000, China; Himalayan Environment Research Institute (HERI), Kathmandu, Nepal.

出版信息

J Environ Sci (China). 2021 Apr;102:37-52. doi: 10.1016/j.jes.2020.09.011. Epub 2020 Sep 28.

DOI:10.1016/j.jes.2020.09.011
PMID:33637262
Abstract

Precipitation represents an important phenomenon for carbon and nitrogen deposition. Here, the concentrations and fluxes of dissolved organic carbon (DOC) and total dissolved nitrogen (TDN) with their potential sources were analyzed in wet precipitation during summer monsoon from the Northern Indo-Gangetic Plain (IGP), important but neglected area. The volume-weighted mean (VWM) concentration of DOC and TDN were 687.04 and 1210.23 µg/L, respectively. Similarly, the VWM concentration of major ions were in a sequence of NH > Ca > SO > Na > K > NO > Cl > Mg > F > NO, suggesting NH and Ca from agricultural activities and crustal dust played a vital role in precipitation chemistry. Moreover, the wet deposition flux of DOC and TDN were 9.95 and 17.06 kg/(ha⋅year), respectively. The wet deposition flux of inorganic nitrogen species such as NH-N and NO-N were 14.31 and 0.47 kg/(ha⋅year), respectively, demonstrating the strong influence of emission sources and precipitation volume. Source attribution from different analysis suggested the influence of biomass burning on DOC and anthropogenic activities (agriculture, animal husbandry) on nitrogenous species. The air-mass back trajectory analysis indicated the influence of air masses originating from the Bay of Bengal, which possibly carried marine and anthropogenic pollutants along with the biomass burning emissions to the sampling site. This study bridges the data gap in the less studied part of the northern IGP region and provides new information for policy makers to deal with pollution control.

摘要

降水是碳氮沉积的重要现象。本研究分析了北印度恒河平原(IGP)季风夏季降水(该地区是一个重要但被忽视的区域)中溶解性有机碳(DOC)和总溶解氮(TDN)及其潜在来源的浓度和通量。DOC 和 TDN 的体积加权平均值(VWM)浓度分别为 687.04 和 1210.23µg/L。同样,主要离子的 VWM 浓度序列为 NH > Ca > SO > Na > K > NO > Cl > Mg > F > NO,表明农业活动和地壳尘埃中的 NH 和 Ca 对降水化学起重要作用。此外,DOC 和 TDN 的湿沉降通量分别为 9.95 和 17.06kg/(ha·年)。NH4-N 和 NO3-N 等无机氮物种的湿沉降通量分别为 14.31 和 0.47kg/(ha·年),表明排放源和降水量的强烈影响。来自不同分析的来源归因表明,生物质燃烧对 DOC 的影响以及人为活动(农业、畜牧业)对含氮物种的影响。空气团后向轨迹分析表明,源自孟加拉湾的空气团的影响,这些空气团可能携带着海洋和人为污染物以及生物质燃烧排放物到达采样点。本研究填补了北 IGP 地区研究较少部分的数据空白,为决策者提供了应对污染控制的新信息。

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