Jiang Mingming, Wan Peng, Tang Kai, Liu Maosheng, Kan Caixia
College of Science, MIIT Key Laboratory of Aerospace Information Materials and Physics, Key Laboratory for Intelligent Nano Materials and Devices, Nanjing University of Aeronautics and Astronautics, No. 29 Jiangjun Road, Nanjing 211106, P. R. China.
Nanoscale. 2021 Mar 18;13(10):5448-5459. doi: 10.1039/d0nr08168j.
Near-infrared micro/nanolaser devices utilizing low-dimensional semiconductors can provide essential building blocks to achieve integrated optoelectronic devices and circuitry for advanced functionalities and are compatible with on-chip technologies. Although significant progress has been made through using narrow-band semiconductor micro/nanostructures to realize near-infrared stimulated radiation at room temperature, severe challenges still remain involving much lower quantum efficiencies and higher auger recombination. Herein, we report an experimental realization of a current-injection semiconductor polariton device made of a ZnO microwire via Ga-doping (ZnO:Ga MW) and p-type GaAs template. The device can emit polaritonic illumination directly from sharp edges of the hexagonal MW. The experimental results of angle-resolved electroluminescence measurements reveal a typical anticrossing feature between excitons and cavity modes, unambiguous evidence of the strong exciton-polariton coupling, with corresponding Rabi splitting energy extracted to be about 195 meV. As the applied bias goes above a certain value, electrically driven whispering gallery lasing action was achieved in the near-infrared spectrum, and the lasing features can be assigned to the exciton-polariton effect. The results not only can afford insights into the development of low-threshold coherent light sources via the exciton-polariton effect, but also can expand the fabrication of low-dimensional, near-infrared microlaser devices.
利用低维半导体的近红外微纳激光器件可为实现具有先进功能的集成光电器件和电路提供关键构建模块,并且与片上技术兼容。尽管通过使用窄带半导体微纳结构在室温下实现近红外受激辐射已取得显著进展,但仍存在严峻挑战,包括量子效率低得多和俄歇复合率更高。在此,我们报告了一种通过Ga掺杂(ZnO:Ga MW)和p型GaAs模板由ZnO微线制成的电流注入半导体极化激元器件的实验实现。该器件可从六边形MW的尖锐边缘直接发射极化激元照明。角分辨电致发光测量的实验结果揭示了激子与腔模之间典型的反交叉特征,这是强激子 - 极化激元耦合的明确证据,提取的相应拉比分裂能量约为195 meV。当施加的偏压超过某个值时,在近红外光谱中实现了电驱动的回音壁激光作用,并且激光特征可归因于激子 - 极化激元效应。这些结果不仅可为通过激子 - 极化激元效应开发低阈值相干光源提供见解,还可扩展低维近红外微激光器件的制造。