Engelhardt Georg, Cao Jianshu
Beijing Computational Science Research Center, Beijing 100193, People's Republic of China.
Department of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, USA.
Phys Rev Lett. 2021 Mar 5;126(9):090601. doi: 10.1103/PhysRevLett.126.090601.
In recent experiments, the light-matter interaction has reached the ultrastrong coupling limit, which can give rise to dynamical generalizations of spatial symmetries in periodically driven systems. Here, we present a unified framework of dynamical-symmetry-protected selection rules based on Floquet response theory. Within this framework, we study rotational, parity, particle-hole, chiral, and time-reversal symmetries and the resulting selection rules in spectroscopy, including symmetry-protected dark states (spDS), symmetry-protected dark bands, and symmetry-induced transparency. Specifically, dynamical rotational and parity symmetries establish spDS and symmetry-protected dark band conditions. A particle-hole symmetry introduces spDSs for symmetry-related Floquet states and also a symmetry-induced transparency at quasienergy crossings. Chiral symmetry and time-reversal symmetry alone do not imply spDS conditions but can be combined to define a particle-hole symmetry. These symmetry conditions arise from destructive interference due to the synchronization of symmetric quantum systems with the periodic driving. Our predictions reveal new physical phenomena when a quantum system reaches the strong light-matter coupling regime, which is important for superconducting qubits, atoms and molecules in optical or plasmonic field cavities, and optomechanical systems.
在最近的实验中,光与物质的相互作用已达到超强耦合极限,这可能会在周期性驱动系统中引发空间对称性的动态推广。在此,我们基于弗洛凯响应理论提出了一个动态对称保护选择规则的统一框架。在这个框架内,我们研究旋转、宇称、粒子 - 空穴、手征和时间反演对称性以及光谱学中由此产生的选择规则,包括对称保护暗态(spDS)、对称保护暗带和对称诱导透明性。具体而言,动态旋转和宇称对称性建立了spDS和对称保护暗带条件。粒子 - 空穴对称性为与对称性相关的弗洛凯态引入了spDS,并且在准能量交叉处还产生了对称诱导透明性。单独的手征对称性和时间反演对称性并不意味着spDS条件,但可以结合起来定义粒子 - 空穴对称性。这些对称条件源于对称量子系统与周期性驱动同步导致的相消干涉。我们的预测揭示了量子系统达到强光 - 物质耦合 regime 时的新物理现象,这对于超导量子比特、光学或等离子体场腔中的原子和分子以及光机械系统非常重要。