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基于低温探测器的实验室扩展X射线吸收精细结构光谱学的可行性。

Feasibility of Laboratory-Based EXAFS Spectroscopy with Cryogenic Detectors.

作者信息

George Simon J, Carpenter Matthew H, Friedrich Stephan, Cantor Robin

机构信息

STAR Cryoelectronics, Santa Fe NM 87508 USA.

Lawrence Livermore National Laboratory, Livermore CA 94550 USA.

出版信息

J Low Temp Phys. 2020 Sep;200(5-6):479-484. doi: 10.1007/s10909-020-02474-7. Epub 2020 Jul 4.

DOI:10.1007/s10909-020-02474-7
PMID:33776141
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7990010/
Abstract

Extended X-ray Absorption Fine Structure (EXAFS) spectroscopy is a powerful technique that gives element-specific information about the structure of molecules. The development of a laboratory EXAFS spectrometer capable of measuring transmission spectra would be a significant advance as the technique is currently only available at synchrotron radiation lightsources. Here, we explore the potential of cryogenic detectors as the energy resolving component of a laboratory transmission EXAFS instrument. We examine the energy resolution, count-rate, and detector stability needed for good EXAFS spectra and compare these to the properties of cryogenic detectors and conventional X-ray optics. We find that superconducting tunnel junction (STJ) detectors are well-suited for this application.

摘要

扩展X射线吸收精细结构(EXAFS)光谱学是一种强大的技术,可提供有关分子结构的元素特异性信息。能够测量透射光谱的实验室EXAFS光谱仪的开发将是一项重大进展,因为该技术目前仅在同步辐射光源上可用。在这里,我们探索了低温探测器作为实验室透射EXAFS仪器的能量分辨组件的潜力。我们研究了获得良好EXAFS光谱所需的能量分辨率、计数率和探测器稳定性,并将这些与低温探测器和传统X射线光学器件的特性进行了比较。我们发现超导隧道结(STJ)探测器非常适合此应用。