Ferrer Brandon R, Gomez-Solano Juan Ruben, Arzola Alejandro V
Instituto de Física, Universidad Nacional Autónoma de México, Ciudad de México, Codigo Postal 04510, México.
Phys Rev Lett. 2021 Mar 12;126(10):108001. doi: 10.1103/PhysRevLett.126.108001.
Thermally activated transitions are ubiquitous in nature, occurring in complex environments which are typically conceived as ideal viscous fluids. We report the first direct observations of a Brownian bead transiting between the wells of a bistable optical potential in a viscoelastic fluid with a single long relaxation time. We precisely characterize both the potential and the fluid, thus enabling a neat comparison between our experimental results and a theoretical model based on the generalized Langevin equation. Our findings reveal a drastic amplification of the transition rates compared to those in a Newtonian fluid, stemming from the relaxation of the fluid during the particle crossing events.
热激活转变在自然界中无处不在,发生在通常被视为理想粘性流体的复杂环境中。我们首次直接观察到一个布朗粒子在具有单一长弛豫时间的粘弹性流体中,在双稳光学势阱之间跃迁。我们精确地表征了势和流体,从而能够将我们的实验结果与基于广义朗之万方程的理论模型进行清晰的比较。我们的研究结果表明,与牛顿流体相比,跃迁速率有显著放大,这源于粒子穿越事件期间流体的弛豫。