Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China.
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China.
J Hazard Mater. 2021 Aug 15;416:125820. doi: 10.1016/j.jhazmat.2021.125820. Epub 2021 Apr 8.
Commodity plastic is ubiquitous in daily life and commonly disposed of via unregulated burning, particularly in developing regions. We report here the much higher emission factors (13.1 ± 7.5 g/kg) and toxicities of inhalable aerosols emitted from the unregulated burning of plastic waste based on field measurements and cellular experiments, including oxidative stress and cytotoxic tests in A549 cells. Plastic foam burning emitted aerosols possesses the highest EFs (34.8 ± 4.5 g/kg) and toxicities, which are 4.2- to 13.4-fold and 1.1- to 2.7-fold higher than those emitted from the burning of other waste types. These quantified toxicities are mainly attributed to aerosols containing carbonaceous matter, especially persistent organic pollutants, including polycyclic aromatic hydrocarbons and dioxins, which originate from incomplete combustion processes. The aerosol emission amounts were estimated from the obtained experimental results. Approximately 70.2 million tons (29%) of plastic waste was burned without regulation worldwide in 2016, leading to 0.92 ± 0.53 million tons of toxic aerosols being released into the air, a majority of which occurred in developing regions. The results indicate improved combustion technology and control strategies are urgently needed in developing regions for discarded plastic -waste to mitigate toxic exposure risks and achieve sustainable development.
商品塑料在日常生活中无处不在,通常通过不受监管的燃烧来处理,尤其是在发展中地区。我们在这里报告了更高的排放因子(13.1±7.5g/kg)和毒性,这些毒性来自于对不可控的塑料废物燃烧的现场测量和细胞实验,包括氧化应激和 A549 细胞的细胞毒性测试。塑料泡沫燃烧产生的气溶胶具有最高的排放因子(34.8±4.5g/kg)和毒性,分别比其他废物类型燃烧产生的气溶胶高出 4.2 到 13.4 倍和 1.1 到 2.7 倍。这些量化的毒性主要归因于含有碳质物质的气溶胶,特别是持久性有机污染物,包括多环芳烃和二恶英,它们来自不完全燃烧过程。气溶胶排放量是根据实验结果估算出来的。2016 年,全球约有 7020 万吨(29%)的塑料废物未经监管燃烧,导致 0.92±0.53 万吨有毒气溶胶释放到空气中,其中大部分发生在发展中地区。研究结果表明,发展中地区急需改进燃烧技术和控制策略,以处理废弃塑料废物,从而减轻有毒物质暴露的风险,实现可持续发展。