Bulgac Aurel, Abdurrahman Ibrahim, Jin Shi, Godbey Kyle, Schunck Nicolas, Stetcu Ionel
Department of Physics, University of Washington, Seattle, Washington 98195-1560, USA.
Cyclotron Institute, Texas A&M University, College Station, Texas 77843, USA.
Phys Rev Lett. 2021 Apr 9;126(14):142502. doi: 10.1103/PhysRevLett.126.142502.
The intrinsic spins and their correlations are the least understood characteristics of fission fragments from both theoretical and experimental points of view. In many nuclear reactions, the emerging fragments are typically excited and acquire an intrinsic excitation energy and an intrinsic spin depending on the type of the reactions and interaction mechanism. Both the intrinsic excitation energies and the fragments' intrinsic spins and parities are controlled by the interaction mechanism and conservations laws, which lead to their correlations and determines the character of their deexcitation mechanism. We outline here a framework for the theoretical extraction of the intrinsic spin distributions of the fragments and their correlations within the fully microscopic real-time density-functional theory formalism and illustrate it on the example of induced fission of ^{236}U and ^{240}Pu, using two nuclear energy density functionals. These fission fragment intrinsic spin distributions display new qualitative features previously not discussed in literature. Within this fully microscopic framework, we extract for the first time the intrinsic spin distributions of fission fragments of ^{236}U and ^{240}Pu as well as the correlations of their intrinsic spins, which have been debated in literature for more than six decades with no definite conclusions so far.
从理论和实验的角度来看,裂变碎片的内禀自旋及其关联是最不为人所理解的特征。在许多核反应中,产生的碎片通常会被激发,并根据反应类型和相互作用机制获得内禀激发能和内禀自旋。内禀激发能以及碎片的内禀自旋和宇称均由相互作用机制和守恒定律控制,这导致了它们之间的关联,并决定了它们的退激机制的特征。在此,我们概述了一个理论框架,用于在完全微观的实时密度泛函理论形式体系内提取碎片的内禀自旋分布及其关联,并以使用两种核能密度泛函的(^{236}U)和(^{240}Pu)诱发裂变为例进行说明。这些裂变碎片的内禀自旋分布展现出此前文献中未讨论过的新的定性特征。在这个完全微观的框架内,我们首次提取了(^{236}U)和(^{240}Pu)裂变碎片的内禀自旋分布以及它们内禀自旋的关联,而关于这些内容,文献中已经争论了六十多年,至今仍没有明确的结论。