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在鼓泡式生物反应器中模拟烃基生物工艺中氧传递系数的定量。

Quantification of oxygen transfer coefficients in simulated hydrocarbon-based bioprocesses in a bubble column bioreactor.

机构信息

DST-NRF Centre of Excellence in Catalysis (c* Change), Pretoria, South Africa.

Department of Process Engineering, Stellenbosch University, Banghoek Road, Stellenbosch, 7600, South Africa.

出版信息

Bioprocess Biosyst Eng. 2021 Sep;44(9):1913-1921. doi: 10.1007/s00449-021-02571-1. Epub 2021 Apr 24.

Abstract

This study investigates the overall volumetric oxygen transfer coefficient (Ka) in multiphase hydrocarbon-based bioprocess under a range of hydrocarbon concentrations (H), solid loadings (deactivated yeast) (S) and superficial gas velocities (U) in a bubble column reactor (BCR). Ka increased with increasing U in the air-water system; due to an increase in the number of small bubbles which enhanced gas holdup. In air-water-yeast systems, the initial addition of yeast increased Ka significantly. Further increases in S reduced Ka, due to increases in the bubble size with increasing S. Ka decreased when H was added in air-water-hydrocarbon systems. However, U, S and H affected Ka differently in air-water-yeast-hydrocarbon systems: an indication of the complex interactions between the yeast and hydrocarbon phases which changed the system's hydrodynamics and therefore affected K. This work illustrates the effect of the operating conditions (S, H and U) on oxygen transfer behaviour in multiphase systems.

摘要

本研究考察了在气泡柱反应器(BCR)中,在一系列烃浓度(H)、固体负荷(失活酵母)(S)和表面气体速度(U)下,多相烃基生物工艺中的总体容积氧转移系数(Ka)。在气-水体系中,Ka 随 U 的增加而增加;这是由于小气泡数量的增加,从而提高了气体持液量。在气-水-酵母体系中,酵母的初始添加显著增加了 Ka。随着 S 的增加,气泡尺寸增大,导致 Ka 降低。在气-水-烃体系中添加 H 时,Ka 会降低。然而,在气-水-酵母-烃体系中,U、S 和 H 对 Ka 的影响不同:这表明酵母相和烃相之间的复杂相互作用改变了系统的流体动力学,从而影响了 K。这项工作说明了操作条件(S、H 和 U)对多相系统中氧传递行为的影响。

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