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电场控制多铁性螺旋磁体中的自然旋光性。

Electric field control of natural optical activity in a multiferroic helimagnet.

机构信息

Department of Applied Physics and Quantum Phase Electronics Center (QPEC), University of Tokyo, Tokyo 113-8656, Japan.

RIKEN Center for Emergent Matter Science (CEMS), Wako, Saitama 351-0198, Japan.

出版信息

Science. 2021 Apr 30;372(6541):496-500. doi: 10.1126/science.aaz4312.

DOI:10.1126/science.aaz4312
PMID:33926951
Abstract

Controlling the chiral degree of freedom in matter has long been an important issue for many fields of science. The spin-spiral order, which exhibits a strong magnetoelectric coupling, gives rise to chirality irrespective of the atomic arrangement of matter. Here, we report the resonantly enhanced natural optical activity on the electrically active magnetic excitation, that is, electromagnon, in multiferroic cupric oxide. The electric field control of the natural optical activity is demonstrated through magnetically induced chirality endowed with magnetoelectric coupling. These optical properties inherent to multiferroics may lead to optical devices based on the control of chirality.

摘要

控制物质中的手性自由度一直是许多科学领域的重要问题。自旋螺旋有序态表现出强烈的磁电耦合,无论物质的原子排列如何,都会产生手性。在这里,我们报告了在多铁性氧化铜中电活性磁激发,即电磁子,的共振增强自然旋光。通过磁电耦合赋予的磁致手性,证明了自然旋光对电场的控制。多铁性固有的这些光学性质可能会导致基于手性控制的光学器件。

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引用本文的文献

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Giant chiral magnetoelectric oscillations in a van der Waals multiferroic.范德瓦尔斯多铁体中的巨大手性磁电振荡。
Nature. 2024 Aug;632(8024):273-279. doi: 10.1038/s41586-024-07678-5. Epub 2024 Jul 17.
2
Terahertz photon to dc current conversion via magnetic excitations of multiferroics.通过多铁性材料的磁激发实现太赫兹光子到直流电流的转换。
Nat Commun. 2024 Jun 6;15(1):4699. doi: 10.1038/s41467-024-49056-9.
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Large nonlinear optical magnetoelectric response in a noncentrosymmetric magnetic Weyl semimetal.非中心对称磁性外尔半金属中的大非线性光学磁电响应。
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Dual-comb optical activity spectroscopy for the analysis of vibrational optical activity induced by external magnetic field.外磁场诱导的振动旋光的双梳光活性光谱分析。
Nat Commun. 2023 Feb 16;14(1):883. doi: 10.1038/s41467-023-36509-w.
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Unconventional interlayer exchange coupling via chiral phonons in synthetic magnetic oxide heterostructures.合成磁性氧化物异质结构中通过手性声子实现的非常规层间交换耦合。
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