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T 型结构各向异性蒸发器用于高性能太阳能驱动零液体排放

Anisotropic Evaporator with a T-Shape Design for High-Performance Solar-Driven Zero-Liquid Discharge.

机构信息

State Key Laboratory of Applied Organic Chemistry, Lanzhou University, Lanzhou, Gansu, 730000, China.

Key Laboratory of Western China's Environmental Systems, College of Earth and Environmental Sciences, Lanzhou University, Lanzhou, Gansu, 730000, China.

出版信息

Small. 2021 Jun;17(24):e2100969. doi: 10.1002/smll.202100969. Epub 2021 May 3.

DOI:10.1002/smll.202100969
PMID:33938137
Abstract

Solar-driven evaporation is regarded as a sustainable wastewater treatment strategy for clean water recovery and salt condensation. However, achieving both high evaporation rate and long-term stability remain challenging due to poor thermal management and rapid salt accumulation and blocking. Here, a T-shape solar-driven evaporator, composed of a surface-carbonized longitudinal wood membrane (C-L-wood) is demonstrated as the top "" for solar harvesting/vapor generation/salt collection and another piece of natural L-wood as the support "" for brine transporting and thermally insulating. The horizontally aligned micro-channels of C-L-wood have a low perpendicular thermal conductivity and can effectively localize the thermal energy for rapid evaporation. Meanwhile, the brine is guided to transport from the support L-wood ("") to the centerline of the top evaporator and then toward the double edge (""), during which clean water is evaporated and salt is crystallized at the edge. The T-shape evaporator demonstrates a high evaporation rate of 2.43 kg m h under 1 sun irradiation, and is stable for 7 days of the outdoor operation, which simultaneously realizes clean water evaporation and salt collection (including Cu , CrO , Co ), and achieves zero-liquid discharge. Therefore, the T-shape design provides an effective strategy for high performance wastewater treatment.

摘要

太阳能驱动蒸发被认为是一种可持续的废水处理策略,可用于清洁水回收和盐浓缩。然而,由于热管理不善以及盐的快速积累和堵塞,实现高蒸发率和长期稳定性仍然具有挑战性。在这里,展示了一种 T 型太阳能蒸发器,由表面碳化的纵向木膜(C-L-wood)作为顶部“”用于太阳能收集/蒸汽生成/盐收集,另一块天然 L-wood 作为支撑“”用于盐水输送和隔热。C-L-wood 的水平排列微通道具有低垂直热导率,可以有效地将热能集中起来实现快速蒸发。同时,盐水从支撑 L-wood(“”)引导到顶部蒸发器的中心线,然后流向双边缘(“”),在此过程中,清水在边缘蒸发,盐结晶。T 型蒸发器在 1 个太阳照射下的蒸发率高达 2.43kg m h ,并且在户外运行 7 天内保持稳定,同时实现了清水蒸发和盐的收集(包括 Cu 、CrO 、Co ),实现了零液体排放。因此,T 型设计为高性能废水处理提供了一种有效的策略。

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