Rössle Matthias, Leitenberger Wolfram, Reinhardt Matthias, Koç Azize, Pudell Jan, Kwamen Christelle, Bargheer Matias
Helmholtz-Zentrum Berlin für Materialien und Energie, Wilhelm-Conrad-Röntgen Campus, BESSY II, Albert-Einstein-Strasse 15, 12489 Berlin, Germany.
Institut für Physik and Astronomie, Universität Potsdam, Karl-Liebknecht-Strasse 24-25, 14476 Potsdam, Germany.
J Synchrotron Radiat. 2021 May 1;28(Pt 3):948-960. doi: 10.1107/S1600577521002484. Epub 2021 Mar 19.
The time-resolved hard X-ray diffraction endstation KMC-3 XPP for optical pump/X-ray probe experiments at the electron storage ring BESSY II is dedicated to investigating the structural response of thin film samples and heterostructures after their excitation with ultrashort laser pulses and/or electric field pulses. It enables experiments with access to symmetric and asymmetric Bragg reflections via a four-circle diffractometer and it is possible to keep the sample in high vacuum and vary the sample temperature between ∼15 K and 350 K. The femtosecond laser system permanently installed at the beamline allows for optical excitation of the sample at 1028 nm. A non-linear optical setup enables the sample excitation also at 514 nm and 343 nm. A time-resolution of 17 ps is achieved with the `low-α' operation mode of the storage ring and an electronic variation of the delay between optical pump and hard X-ray probe pulse conveniently accesses picosecond to microsecond timescales. Direct time-resolved detection of the diffracted hard X-ray synchrotron pulses use a gated area pixel detector or a fast point detector in single photon counting mode. The range of experiments that are reliably conducted at the endstation and that detect structural dynamics of samples excited by laser pulses or electric fields are presented.
用于电子储存环BESSY II上光泵浦/X射线探测实验的时间分辨硬X射线衍射终端站KMC-3 XPP,致力于研究薄膜样品和异质结构在受到超短激光脉冲和/或电场脉冲激发后的结构响应。它通过四圆衍射仪实现对对称和非对称布拉格反射的实验,并且能够将样品保持在高真空环境中,并在约15 K至350 K之间改变样品温度。永久安装在该光束线上的飞秒激光系统可在1028 nm波长下对样品进行光激发。非线性光学装置还能在514 nm和343 nm波长下实现样品激发。利用储存环的“低α”运行模式可实现17 ps的时间分辨率,通过光泵浦和硬X射线探测脉冲之间延迟的电子调节,方便地进入皮秒到微秒的时间尺度。对衍射的硬X射线同步辐射脉冲的直接时间分辨检测采用门控面积像素探测器或单光子计数模式下的快速点探测器。本文介绍了在该终端站可靠进行的、检测由激光脉冲或电场激发的样品结构动力学的一系列实验。