Zhang Wenjun, Zhang Yuquan, Zhang Shuoshuo, Wang Yulong, Yang Wu, Min Changjun, Yuan Xiaocong
Opt Express. 2021 Apr 12;29(8):11664-11673. doi: 10.1364/OE.422493.
Surface plasmon optical tweezers based on micro- and nano-structures are capable of capturing particles in a very small spatial scale and have been widely used in many front research fields. In general, distribution of optical forces and potential wells exerted on the particles can be modulated by controlling the geometric parameters of the structures. However, these fabricated structures are irreversible once processed, which greatly limits its application in dynamic manipulation. The plasmonic field in these structures can be enhanced with orders of magnitude compared to the excitation light, offering a possibility to stimulate nonlinear responses as a new degree of freedom for dynamic modulation. Here, we theoretically demonstrate that the optical force and potential well can be modulated on account of the nonlinear Kerr effect of a gold bowtie structure under a pulsed laser with high peak power. The results verify that the trapping states, including the position, width, and depth of the potential well, can be dynamically modulated by changing intensity of the incident laser. It provides an effective approach for stable trapping and dynamic controlling of particles on nanostructure-based plasmonic trapping platforms and thus has great application potential in many fields, such as enhanced Raman detection, super-resolution imaging, and optical sensing.
基于微纳结构的表面等离子体光镊能够在非常小的空间尺度内捕获粒子,并且已经在许多前沿研究领域中得到广泛应用。一般来说,通过控制结构的几何参数,可以调制施加在粒子上的光力和势阱分布。然而,这些制造出来的结构一旦加工完成就不可逆转,这极大地限制了其在动态操纵方面的应用。与激发光相比,这些结构中的等离子体场可以增强几个数量级,这为激发非线性响应提供了可能性,作为动态调制的一个新自由度。在这里,我们从理论上证明,在具有高峰值功率的脉冲激光作用下,由于金蝴蝶结结构的非线性克尔效应,光力和势阱可以被调制。结果证实,包括势阱的位置、宽度和深度在内的捕获状态可以通过改变入射激光的强度来动态调制。它为基于纳米结构的等离子体捕获平台上的粒子稳定捕获和动态控制提供了一种有效方法,因此在许多领域具有巨大的应用潜力,如增强拉曼检测、超分辨率成像和光学传感。