School of Mechanical and Automotive Engineering, Shanghai University of Engineering Science, Shanghai 201620, China.
School of Mechanical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China.
J Environ Sci (China). 2021 Jun;104:326-334. doi: 10.1016/j.jes.2020.12.005. Epub 2020 Dec 28.
This paper presents detailed measurements of gaseous species during the reburning process with high CO concentration in a bench-scale furnace. Superfine pulverized coal, with the average particle size below or around 20 μm, is used as the reburning fuel. The data of flue gas concentration (NO, HCN, NH, CH, O, CO, CO etc.) is obtained in order to reveal the intrinsic connection between NO emissions and other influential gaseous species at different positions of the furnace. The finding concludes that the advantage of superfine pulverized coal with regard to NO reduction is more efficient in homogeneous stage rather than heterogeneous stage. Meanwhile, the evolution of HCN and CH agrees well with each stage of NO reduction, which indicates that these gaseous species are favorable for NO abatement. Eventually, oxygen consumption rate for superfine pulverized coal is relatively faster, conducive to strengthen both homogeneous and heterogeneous NO reduction under CO reburning condition.
本文在台架炉中采用高浓度 CO 条件下详细测量了再燃过程中的气态物质。超细煤粉(平均粒径在 20μm 以下或左右)被用作再燃燃料。获得了烟道气浓度(NO、HCN、NH、CH、O、CO、CO 等)的数据,以揭示不同炉膛位置NO 排放与其他有影响的气态物质之间的内在联系。研究结果表明,超细煤粉在均相阶段而非非均相阶段对 NO 减排的优势更为显著。同时,HCN 和 CH 的演变与 NO 减排的各个阶段都很好地吻合,这表明这些气态物质有利于 NO 的去除。最终,超细煤粉的耗氧速率相对较快,有利于在 CO 再燃条件下强化均相和非均相的 NO 还原。