Caridad José M, Tserkezis Christos, Santos Jaime E, Plochocka Paulina, Venkatesan Munuswamy, Coey J M D, Mortensen N Asger, Rikken Geert L J A, Krstić Vojislav
School of Physics, CRANN, Amber Research Centre, Trinity College Dublin, College Green, Dublin 2, Ireland.
DTU Physics, Technical University of Denmark, 2800 Kongens Lyngby, Denmark.
Phys Rev Lett. 2021 Apr 30;126(17):177401. doi: 10.1103/PhysRevLett.126.177401.
The connection between chirality and electromagnetism has attracted much attention through the recent history of science, allowing the discovery of crucial nonreciprocal optical phenomena within the context of fundamental interactions between matter and light. A major phenomenon within this family is the so-called Faraday chiral anisotropy, the long-predicted but yet unobserved effect which arises due to the correlated coaction of both natural and magnetically induced optical activities at concurring wavelengths in chiral systems. Here, we report on the detection of the elusive anisotropic Faraday chiral phenomenon and demonstrate its enantioselectivity. The existence of this fundamental effect reveals the accomplishment of envisioned nonreciprocal electromagnetic metamaterials referred to as Faraday chiral media, systems where novel electromagnetic phenomena such as negative refraction of light at tunable wavelengths or even negative reflection can be realized. From a more comprehensive perspective, our findings have profound implications for the general understanding of parity-violating photon-particle interactions in magnetized media.
在手性与电磁学之间的联系在近代科学史上备受关注,这使得人们能够在物质与光的基本相互作用背景下发现关键的非互易光学现象。这一类别中的一个主要现象是所谓的法拉第手性各向异性,这是一种长期以来被预测但尚未观测到的效应,它是由于手性系统中在相同波长下自然光学活性和磁致光学活性的相关共同作用而产生的。在此,我们报告了对难以捉摸的各向异性法拉第手性现象的检测,并展示了其对映选择性。这种基本效应的存在揭示了被称为法拉第手性介质的预期非互易电磁超材料的实现,在这种系统中可以实现诸如可调波长下光的负折射甚至负反射等新型电磁现象。从更全面的角度来看,我们的发现对于深入理解磁化介质中违反宇称的光子 - 粒子相互作用具有深远意义。