Zhang Qiang, Liu Zhirong, Cheng Ziqiang
Department of Applied Physics, East China Jiaotong University, Nanchang 330013, China.
Nanomaterials (Basel). 2023 Aug 4;13(15):2251. doi: 10.3390/nano13152251.
The coupling of the spin-orbit angular momentum of photons in a focused spatial region can enhance the localized optical field's chirality. In this paper, a scheme for producing a superchiral optical field in a 4π microscopic system is presented by tightly focusing two counter-propagating spiral wavefronts. We calculate the optical forces and torques exerted on a chiral dipole by the chiral light field and reveal the chiral forces by combining the light field and dipoles. Results indicate that, in addition to the general optical force, particles' motion would be affected by a chiral force that is directly related to the particle chirality. This chiral mechanical effect experienced by the electromagnetic dipoles excited on a chiral particle could be characterized by the behaviors of chirality density and flux, which are, respectively, associated with the reactive and dissipative components of the chiral forces. This work facilitates the advancement of optical separation and manipulation techniques for chiral particles.
聚焦空间区域中光子的自旋 - 轨道角动量耦合可以增强局域光场的手性。本文提出了一种在4π微观系统中通过紧密聚焦两个反向传播的螺旋波前产生超手性光场的方案。我们计算了手性光场对手性偶极子施加的光学力和扭矩,并通过结合光场和偶极子揭示了手性力。结果表明,除了一般的光学力外,粒子的运动还会受到与粒子手性直接相关的手性力的影响。手性粒子上激发的电磁偶极子所经历的这种手性力学效应可以通过手性密度和通量的行为来表征,它们分别与手性力的无功和耗散分量相关。这项工作促进了手性粒子的光学分离和操纵技术的发展。