Suppr超能文献

可见光驱动的 BiMoO-rGO-TiO 光催化剂的构建及其对氧氟沙星的有效降解。

Construction of visible-light driven BiMoO-rGO-TiO photocatalyst for effective ofloxacin degradation.

机构信息

Department of Chemistry, College of Natural Sciences, Yeungnam University, Gyeongsan, Gyeongbuk, 38541, Republic of Korea.

Department of Chemistry, College of Natural Sciences, Yeungnam University, Gyeongsan, Gyeongbuk, 38541, Republic of Korea.

出版信息

Environ Res. 2021 Aug;199:111261. doi: 10.1016/j.envres.2021.111261. Epub 2021 May 17.

Abstract

Photocatalytic removal is more appropriate for the destruction of organic contaminants. The ternary BiMoO-reduced graphene oxide (rGO)-TiO catalyst was synthesized using a simple hydrothermal method, and various surface analytical optical techniques were analyzed. The photocatalytic decomposition efficiency of the BiMoO-rGO-TiO composite was 92.3% higher than those of pure and binary photocatalysts. The effects of operational parameters, such as catalyst ratio, catalyst variation, rGO ratio variation, and pH value variation were also analyzed. The as-prepared ternary photocatalyst exhibited low photoluminescence and high photocurrent density, which suppressed photon-induced electron and hole (h) recombination and effective charge separation. The study demonstrated that rGO has excellent electron transfer performance and enhanced photocatalytic reaction stability. The perfect cycling stability of BiMoO-rGO-TiO was retained even after five consecutive cycles on the photocatalytic degradation reaction performance. In this study, we propose a decomposition performance mechanism for ofloxacin degradation that underwent visible-light irradiation.

摘要

光催化去除更适合于有机污染物的破坏。采用简单的水热法合成了三元 BiMoO-还原氧化石墨烯(rGO)-TiO 催化剂,并对其进行了各种表面分析光学技术分析。BiMoO-rGO-TiO 复合光催化剂的光催化分解效率比纯相和二元光催化剂分别提高了 92.3%。还分析了操作参数,如催化剂比例、催化剂变化、rGO 比例变化和 pH 值变化的影响。所制备的三元光催化剂表现出低的光致发光和高的光电流密度,抑制了光子诱导电子和空穴(h)复合和有效的电荷分离。研究表明,rGO 具有优异的电子传输性能和增强的光催化反应稳定性。即使在光催化降解反应性能上连续进行五次循环后,BiMoO-rGO-TiO 的完美循环稳定性仍然得以保留。在本研究中,我们提出了一个光降解机制,用于研究氧氟沙星的可见光照射下的降解性能。

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验