Zhu Shengqiang, Poetzscher James, Shen Juanyong, Wang Siyu, Wang Peng, Zhang Hongliang
Department of Environmental Science and Engineering Fudan University Shanghai China.
School of Environmental Science and Engineering Nanjing University of Information Science and Technology Nanjing China.
Geophys Res Lett. 2021 May 28;48(10):e2021GL093668. doi: 10.1029/2021GL093668. Epub 2021 May 18.
Economic activities and the associated emissions have significantly declined during the 2019 novel coronavirus (COVID-19) pandemic, which has created a natural experiment to assess the impact of the emitted precursor control policy on ozone (O) pollution. In this study, we utilized comprehensive satellite, ground-level observations, and source-oriented chemical transport modeling to investigate the O variations during the COVID-19 pandemic in China. Here, we found that the significant elevated O in the North China Plain (40%) and Yangtze River Delta (35%) were mainly attributed to the enhanced atmospheric oxidation capacity (AOC) in these regions, associated with the meteorology and emission reduction during lockdown. Besides, O formation regimes shifted from VOC-limited regimes to NO-limited and transition regimes with the decline of NO during lockdown. We suggest that future O control policies should comprehensively consider the effects of AOC on the O elevation and coordinated regulations of the O precursor emissions.
在2019年新型冠状病毒(COVID-19)大流行期间,经济活动及相关排放显著下降,这创造了一个天然实验,以评估排放前体控制政策对臭氧(O₃)污染的影响。在本研究中,我们利用综合卫星、地面观测以及源导向化学传输模型,来研究中国COVID-19大流行期间的O₃变化。在此,我们发现,华北平原(40%)和长江三角洲(35%)的O₃显著升高,主要归因于这些地区大气氧化能力(AOC)的增强,这与封锁期间的气象条件和减排有关。此外,随着封锁期间NO的减少,O₃生成机制从VOC限制机制转变为NO限制和过渡机制。我们建议,未来的O₃控制政策应全面考虑AOC对O₃升高的影响以及对O₃前体排放的协同监管。