Chen Yuxuan, He Yuhang, Zhang Yifan, Tian Zhen, Dai Jianming
Opt Express. 2021 Jun 21;29(13):20477-20486. doi: 10.1364/OE.425207.
Understanding the process of terahertz (THz) wave generation from liquid water is crucial for further developing liquid THz sources. We present a systematic investigation of THz wave generated from laser-irradiated water lines. We show that water line in the diameter range of 0.1-0.2 mm generates the strongest THz wave, and THz frequency red shift is observed when diameter of the water line increases. The pump pulse energy dependence is decoupled from self-focusing effect by compensating the focal point displacement. As the pump pulse energy increases, saturation effect in THz peak electric field is observed, which can be mainly attributed to the intensity clamping effect inside the plasma and have never been reported previously, using water line or water film as the THz source. The proposed mechanism for saturation is supported by an independent measurement of laser pulse spectrum broadening. This work may help to further understand the laser-liquid interaction in THz generation process.
了解从液态水产生太赫兹(THz)波的过程对于进一步开发液态太赫兹源至关重要。我们对激光辐照水线产生的太赫兹波进行了系统研究。我们发现直径在0.1 - 0.2毫米范围内的水线产生最强的太赫兹波,并且当水线直径增加时会观察到太赫兹频率红移。通过补偿焦点位移,泵浦脉冲能量依赖性与自聚焦效应解耦。随着泵浦脉冲能量增加,在太赫兹峰值电场中观察到饱和效应,这主要可归因于等离子体内的强度钳制效应,并且以前使用水线或水膜作为太赫兹源时从未报道过。通过对激光脉冲光谱展宽的独立测量支持了所提出的饱和机制。这项工作可能有助于进一步理解太赫兹产生过程中的激光 - 液体相互作用。