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在氟化钙中实现高重复率绿光抽运超连续谱产生。

High repetition rate green-pumped supercontinuum generation in calcium fluoride.

机构信息

Laser Research Center, Vilnius University, Saulėtekio Avenue 10, LT, 10223, Vilnius, Lithuania.

出版信息

Sci Rep. 2021 Jul 22;11(1):15019. doi: 10.1038/s41598-021-94411-1.

Abstract

We compare supercontinuum generation in [Formula: see text] crystal under tight and loose focusing of 150 fs, 515 nm second harmonic pulses from an amplified Yb:KGW laser at a repetition rate of 10 kHz. It is demonstrated that supercontinuum generation geometry applying loose focusing ([Formula: see text]) of the pump beam into a long (25 mm) [Formula: see text] sample is advantageous in terms of supercontinuum spectral extent and durability of damage-free operation of the nonlinear material as compared to a commonly used supercontinuum generation setup which employs tight focusing ([Formula: see text]) into a short (5 mm) sample and to setup which uses tight focusing into a long (25 mm) sample. More specifically, loose focusing into a long sample showed remarkably longer (20 min) damage-free operation of the nonlinear material, which was not translated with respect of the pump beam, while in tight focusing condition the sample is damaged just within 2 min of operation, leading to a complete extinction of the supercontinuum spectrum. The evolution of optical degradation of the nonlinear material in time and its impact to supercontinuum spectrum is studied in terms of filament-induced luminescence due to self-trapped exciton emission and light scattering at the pump wavelength indicating the onset of optical damage. Our findings are supported by the numerical simulations which compare relevant parameters related to filament propagation in tight and loose focusing conditions.

摘要

我们比较了在 10 kHz 重复率的放大 Yb:KGW 激光的 150 fs、515nm 二次谐波脉冲的紧聚焦和松聚焦条件下[公式:见文本]晶体中的超连续谱产生。结果表明,与通常使用的将泵浦光束紧聚焦[公式:见文本]到短(5 毫米)[公式:见文本]样品中的超连续谱产生设置相比,将泵浦光束松聚焦[公式:见文本]到长(25 毫米)[公式:见文本]样品中有利于超连续谱光谱范围和非线性材料无损伤操作的耐久性。更具体地说,将长样品松聚焦显示出明显更长(20 分钟)的无损伤非线性材料操作,而在紧聚焦条件下,样品在 2 分钟的操作内就会损坏,导致超连续谱完全消失。通过自陷激子发射的细丝诱导发光和在泵浦波长处的光散射,研究了非线性材料的光降解随时间的演变及其对超连续谱的影响,表明了光学损伤的开始。我们的发现得到了数值模拟的支持,这些模拟比较了紧聚焦和松聚焦条件下细丝传播的相关参数。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e605/8298603/75c94112f9c0/41598_2021_94411_Fig1_HTML.jpg

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