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中国北方巴丹吉林沙漠浅层地下水和湖水的锶同位素及水化学特征。

Strontium isotopic and hydrochemical characteristics of shallow groundwater and lake water in the Badain Jaran Desert, North China.

机构信息

Chongqing Branch, Changjiang River Scientific Research Institute, Chongqing, People's Republic of China.

Institute of Earth Critical Zone, College of Earth Sciences and Engineering, Jiangning Campus of Hohai University, Nanjing, People's Republic of China.

出版信息

Isotopes Environ Health Stud. 2021 Oct;57(5):516-534. doi: 10.1080/10256016.2021.1961766. Epub 2021 Aug 4.

DOI:10.1080/10256016.2021.1961766
PMID:34347540
Abstract

Shallow groundwater and lake water are the dominant water resources in the Badain Jaran Desert. There are still controversial hypotheses related to the origin of groundwater in this desert. Few studies have been conducted to explore the Sr provenance of these waters and assess the water-rock interactions using a Sr isotope approach until now. In this text, the Sr isotope data of waters in the hinterland of the Badain Jaran Desert and neighbouring areas are reported. The waters in the Badain Jaran Desert have few links to its surrounding rivers, but could be influenced by the precipitation in the Yabulai Mountains. The Sr/Sr ratio changes constantly, while the Sr concentration of shallow groundwater gradually decreases from Yabulai to the desert hinterland to Gurinai-Guaizihu. Combined with hydrochemical data and hydrodynamic conditions, these results show that the dissolved Sr of waters in the desert hinterland is controlled by the Yabulai precipitation and catchment weathering. They further show that the desert shallow groundwater Sr originates mainly from the Yabulai precipitation (> 94 %), while whole-rock weathering contributes little (< 6 %), as calculated using isotope mass balance equations. Relative Sr contributions to lakes from shallow groundwater and catchment weathering are calculated to be 92.5 and 7.5 %, respectively.

摘要

浅层地下水和湖泊水是巴丹吉林沙漠的主要水资源。关于该沙漠地下水的成因,仍存在一些有争议的假说。直到现在,很少有研究利用 Sr 同位素方法来探讨这些水的 Sr 来源,并评估水-岩相互作用。本文报道了巴丹吉林沙漠腹地及周边地区水的 Sr 同位素数据。巴丹吉林沙漠的水与周围的河流联系较少,但可能受到雅布赖山降水的影响。Sr/Sr 比值不断变化,而浅层地下水的 Sr 浓度从雅布赖山到沙漠腹地再到古日乃-拐子湖逐渐降低。结合水化学数据和水动力条件,这些结果表明,沙漠腹地水的溶解 Sr 受雅布赖山降水和集水区风化作用的控制。它们进一步表明,沙漠浅层地下水 Sr 主要来源于雅布赖山降水(>94%),而全岩风化作用的贡献较小(<6%),这是通过同位素质量平衡方程计算得出的。根据同位素质量平衡方程计算得出,浅层地下水和集水区风化对湖泊 Sr 的相对贡献分别为 92.5%和 7.5%。

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