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强耦合手性量子发射器等离子体纳米结构中的定向能量传输

Directional energy transport in strongly coupled chiral quantum emitter plasmonic nanostructures.

作者信息

Gettapola Kamani, Gunapala Sarath D, Premaratne Malin

机构信息

Advanced Computing and Simulation Laboratory (AχL), Department of Electrical and Computer Systems Engineering, Monash University, Clayton, Victoria 3800, Australia.

Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA 91109, United States of America.

出版信息

J Phys Condens Matter. 2021 Sep 8;33(47). doi: 10.1088/1361-648X/ac203f.

Abstract

Achieving directional exciton energy transport can revolutionize a plethora of applications that depend on exciton energy transfer. In this study, we theoretically analyse a system that comprises a collection of chiral quantum emitters placed in a plasmonic setup made up of a metal nanoparticle trimer. We investigate the system by pumping left and right circularly polarized photons to excite the system. We observe that the generated localized surface plasmon modes are polarization-depended, causing chiral coupling between the quantum emitters and the plasmon optical modes. Based on the plasmon field intensity profiles, we show that directional exciton transport can be obtained when the light-matter interaction becomes adequately strong, leading the system towards the strong coupling regime.

摘要

实现定向激子能量传输能够彻底改变众多依赖激子能量转移的应用。在本研究中,我们从理论上分析了一个系统,该系统由置于由金属纳米颗粒三聚体构成的等离子体装置中的手性量子发射器集合组成。我们通过泵浦左旋和右旋圆偏振光子来激发该系统,从而对其进行研究。我们观察到,所产生的局域表面等离子体模式取决于偏振,从而在量子发射器与等离子体光学模式之间引起手性耦合。基于等离子体场强分布,我们表明,当光与物质的相互作用变得足够强时,能够实现定向激子传输,使系统趋向强耦合 regime。 (注:这里“regime”未找到准确对应中文词汇,保留英文)

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