School of Environmental and Municipal Engineering, Qingdao University of Technology, Qingdao 266033, PR China.
College of Oceanic and Atmospheric Sciences, Ocean University of China, Qingdao 266100, PR China.
J Hazard Mater. 2021 Aug 15;416:125833. doi: 10.1016/j.jhazmat.2021.125833. Epub 2021 Apr 20.
Aerosol emissions from wastewater treatment plants (WWTPs) have been associated with health reverberation but studies about characteristics of size-segregated aerosol particulate matter (PM) are scarce. In this study, the measurement of particulate number size distribution in the range of < 10 µm, and the collection of PM, PM and PM, were conducted from an aerobic moving bed biofilm reactor (MBBR) at a full-scale WWTP. MBBR aerosols showed a unimodal number size distribution, with the majority of particles (>94%) in the ultrafine size range (<100 nm). For toxic metal(loid)s or potential pathogens, significant differences were found within MBBR aerosols (PM, PM, and PM), and also between MBBR aerosols and wastewater. Both wastewater and ambient air had important source contributions for MBBR aerosols. The compositions of toxic metal(loid)s in PM, and the populations of potential bacterial or fungal pathogens in PM and PM, were dominated by that from wastewater. Compared to PM and PM, PM had the highest aerosolization potential for the toxic metal(loid)s of As, Cd, Co, Cr, Li, Mn, Ni, U, and Zn, and the genera of Acinetobacter, Pseudomonas and Fusarium. Due to the size-segregated specialty, targeted measures should be employed to reduce the health risks. CAPSULE: The compositions of toxic metal(loid)s in PM, and the populations of potential pathogens in PM and PM, were dominated by that from wastewater.
污水处理厂(WWTP)的气溶胶排放与健康影响有关,但关于大小分级气溶胶颗粒物(PM)特征的研究很少。在这项研究中,从一个全规模的好氧移动床生物膜反应器(MBBR)中测量了 <10 µm 范围内的颗粒物数量粒径分布,并收集了 PM、PM 和 PM。MBBR 气溶胶呈单峰数量粒径分布,大多数颗粒(>94%)处于超细粒径范围(<100nm)。对于有毒金属(loid)或潜在的病原体,在 MBBR 气溶胶(PM、PM 和 PM)内以及在 MBBR 气溶胶和废水之间都发现了显著差异。废水和环境空气对 MBBR 气溶胶都有重要的来源贡献。PM 中的有毒金属(loid)的组成,以及 PM 和 PM 中的潜在细菌或真菌病原体的种群,主要来自废水。与 PM 和 PM 相比,PM 对 As、Cd、Co、Cr、Li、Mn、Ni、U 和 Zn 等有毒金属(loid)以及不动杆菌属、假单胞菌属和镰刀菌属的气溶胶化潜力最高。由于粒径分级的特点,应采取有针对性的措施来降低健康风险。
注:PM 中的有毒金属(loid)的组成,以及 PM 和 PM 中的潜在细菌或真菌病原体的种群,主要来自废水。