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由局限于薄系统中的哑铃状单斑块粒子形成的团簇。

Clusters formed by dumbbell-like one-patch particles confined in thin systems.

作者信息

Sato Masahide

机构信息

Emerging Media Initiative, Kanazawa University, Kanazawa, 920-1192, Japan.

出版信息

Sci Rep. 2021 Sep 10;11(1):18078. doi: 10.1038/s41598-021-97542-7.

Abstract

Performing isothermal-isochoric Monte Carlo simulations, I examine the types of clusters that dumbbell-like one-patch particles form in thin space between two parallel walls, assuming that each particle is synthesized through the merging of two particles, one non-attracting and the other attracting for which, for example, the inter-particle interaction is approximated by the DLVO model . The shape of these dumbbell-like particles is controlled by the ratio of the diameters q of the two spherical particles and by the dimensionless distance l between these centers. Using a modified Kern-Frenkel potential, I examine the dependence of the cluster shape on l and q. Large island-like clusters are created when [Formula: see text]. With increasing q, the clusters become chain-like . When q increases further, elongated clusters and regular polygonal clusters are created. In the simulations, the cluster shape becomes three-dimensional with increasing l because the thickness of the thin system increases proportionally to l.

摘要

通过进行等温等容蒙特卡罗模拟,我研究了哑铃状单斑块粒子在两个平行壁之间的薄空间中形成的团簇类型,假设每个粒子是由两个粒子合并而成,一个无吸引力,另一个有吸引力,例如,粒子间相互作用由DLVO模型近似。这些哑铃状粒子的形状由两个球形粒子的直径比q以及它们中心之间的无量纲距离l控制。使用修正的Kern-Frenkel势,我研究了团簇形状对l和q的依赖性。当[公式:见原文]时会形成大的岛状团簇。随着q的增加,团簇变得像链状。当q进一步增加时,会形成细长团簇和规则多边形团簇。在模拟中,随着l的增加,团簇形状变为三维,因为薄系统的厚度与l成比例增加。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce29/8433354/2175ce661959/41598_2021_97542_Fig1_HTML.jpg

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