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中国北方特大城市天津街道尘埃中有机紫外吸收剂的浓度、分布及潜在健康风险

Concentrations, distribution and potential health risks of organic ultraviolet absorbents in street dust from Tianjin, a megacity in northern China.

机构信息

Key Laboratory of Ecology and Environment in Minority Areas (Minzu University of China), National Ethnic Affairs Commission, Beijing, 100081, China; College of Life and Environmental Sciences, Minzu University of China, Beijing, 100081, China.

College of Environmental Science and Engineering, North China Electric Power University, Beijing, 102206, China.

出版信息

Environ Res. 2022 Mar;204(Pt B):112130. doi: 10.1016/j.envres.2021.112130. Epub 2021 Sep 25.

Abstract

The distribution of organic ultraviolet absorbers (OUVAs) in outdoor dust remains poorly understood, especially in megacities. We measured the concentrations of 11 OUVAs in street dust from Tianjin, China, by a gas chromatography-mass spectrometry, and found total concentrations in the range of 10.3-129 ng/g. These OUVAs were prevalent in the study street dust, but their concentrations were much lower than those in indoor dust reported in other areas previously. Benzophenone and octocrylene were the dominant OUVAs, representing medians of 15.5% and 13.1% of total OUVA concentrations, respectively. Total concentrations of dust OUVAs in the industrial area were higher than the residential, cultural and new urban areas. Source assessment indicated that the OUVAs likely originated mainly from the manufacture and consumption of cosmetics and personal care products, and some may have been from the production and use of OUVA-containing consumer products. The calculated non-carcinogenic risks of OUVAs in street dust were low. Our results further confirmed that the OUVAs were prevalent in the environment, provide useful information for understanding potential risks of these chemicals and developing risk management strategies. Further studies are needed to investigate the occurrence, environmental behaviors and potential risks of these emerging contaminants in outdoor environment.

摘要

户外灰尘中有机紫外线吸收剂(OUVA)的分布仍知之甚少,尤其是在特大城市。我们采用气相色谱-质谱法测量了来自中国天津街道灰尘中 11 种 OUVAs 的浓度,发现其总浓度在 10.3-129ng/g 范围内。这些 OUVAs 在研究街道灰尘中普遍存在,但浓度远低于以前在其他地区报告的室内灰尘中的浓度。二苯甲酮和奥克立林是主要的 OUVAs,分别占总 OUVA 浓度中位数的 15.5%和 13.1%。工业区的灰尘 OUVAs 总浓度高于住宅、文化和新城区。来源评估表明,这些 OUVAs 可能主要来自化妆品和个人护理产品的制造和消费,一些可能来自含有 OUVAs 的消费产品的生产和使用。街道灰尘中 OUVAs 的非致癌风险较低。我们的研究结果进一步证实了 OUVAs 在环境中普遍存在,为了解这些化学物质的潜在风险和制定风险管理策略提供了有用的信息。需要进一步研究以调查这些新兴污染物在户外环境中的发生、环境行为和潜在风险。

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