Suppr超能文献

外加磁场中磁活性超球的流动和分离。

Flux and separation of magneto-active superballs in applied fields.

机构信息

University of Vienna, Physics Faculty/Research Platform MMM Mathematics-Magnetism-Materials, Vienna, Austria.

Faculty of Physics, University of Vienna, Boltzmanngasse 5, 1090 Vienna, Austria.

出版信息

Phys Chem Chem Phys. 2021 Oct 27;23(41):23827-23835. doi: 10.1039/d1cp03343c.

Abstract

The term "active matter" describes a class of out-of-equilibrium systems, whose ability to transform environmental to kinetic energy is sought after in multiple fields of science. A challenge that still remains is to craft nanometer-sized active particles, whose motion can be efficiently directed by externally applied bio-noninvasive stimuli. Adding a magnetic component and therefore being able to direct the motion of active nanoparticles with an applied magnetic field is one of the promising solutions in the field. In this study, we employ molecular dynamics simulations to predict an external field-induced flow that arises in mixtures of magneto-active nanosized cubic and spherical particles with distinct mutual orientations between magnetization and propulsion. We explain why the flux of the suspended particles in the field direction does not only depend on the angle between the active force, driving a particle forward, and the orientation of its magnetization, but also on particle shape and inter-particle interactions. Our results show that by tuning those parameters, one can achieve complete separation of particles according to their magnetization orientation. Based on our findings, along with optimizing the cargo properties of magneto-active nano-units, the actual composition of the magneto-active particle suspension can be characterized.

摘要

“活性物质”这一术语描述了一类非平衡系统,其将环境能量转化为动能的能力在多个科学领域都受到了广泛关注。目前仍然面临的挑战是制造纳米级的活性粒子,这些粒子的运动可以通过外部施加的生物非侵入性刺激来有效地控制。添加磁性组件并因此能够通过施加磁场来控制活性纳米粒子的运动是该领域的一个很有前途的解决方案。在这项研究中,我们采用分子动力学模拟来预测在磁活性纳米立方和球形粒子混合物中出现的外场诱导流,这些粒子在磁化和推进方面具有不同的相互取向。我们解释了为什么悬浮粒子在磁场方向上的通量不仅取决于驱动粒子向前的主动力与粒子磁化方向之间的夹角,还取决于粒子形状和粒子间相互作用。我们的研究结果表明,通过调整这些参数,可以根据粒子的磁化方向实现完全的粒子分离。基于我们的发现,并优化磁活性纳米单元的货物特性,可以对磁活性粒子悬浮液的实际成分进行表征。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9ab4/8549445/4c04ff3554e6/d1cp03343c-f1.jpg

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验