Reichert Julian, Mandal Suvendu, Voigtmann Thomas
Institut für Materialphysik im Weltraum, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 51170 Köln, Germany.
Department of Physics, Heinrich-Heine Universität Düsseldorf, Universitätsstrasse 1, 40225 Düsseldorf, Germany.
Phys Rev E. 2021 Oct;104(4-1):044608. doi: 10.1103/PhysRevE.104.044608.
We derive a mode-coupling theory (MCT) to describe the dynamics of a tracer particle that is embedded in a dense system of active Brownian particles (ABPs) in two spatial dimensions. The ABP undergo translational and rotational Brownian motion and are equipped with a fixed self-propulsion speed along their orientational vector that describes their active motility. The resulting equations of motion for the tagged-particle density-correlation functions describe the various cases of tracer dynamics close to the glass transition: that of a single active particle in a glass-forming passive host suspensions, that of a passive colloidal particle in a suspension of ABP, and that of active tracers in a bath of active particles. Numerical results are presented for these cases assuming hard-sphere interactions among the particles. The qualitative and quantitative accuracy of the theory is tested against event-driven Brownian dynamics (ED-BD) simulations of active and passive hard disks. Simulation and theory are found in quantitative agreement, provided one adjusts the overall density (as known from the passive description of glassy dynamics), and allows for a rescaling of self-propulsion velocities in the active host system. These adjustments account for the fact that ABP-MCT generally overestimates the tendency for kinetic arrest. We confirm in the simulations a peculiar feature of the transient and stationary dynamical density-correlation functions regarding their lack of symmetry under time reversal, demonstrating the nonequilibrium nature of the system and how it manifests itself in the theory.
我们推导了一种模式耦合理论(MCT),以描述嵌入二维空间中密集活性布朗粒子(ABP)系统的示踪粒子的动力学。ABP经历平移和旋转布朗运动,并沿其描述主动运动性的取向矢量配备固定的自推进速度。标记粒子密度相关函数的运动方程描述了接近玻璃化转变的示踪动力学的各种情况:在形成玻璃的被动主体悬浮液中的单个活性粒子的情况、在ABP悬浮液中的被动胶体粒子的情况以及在活性粒子浴中的活性示踪剂的情况。针对这些情况给出了假设粒子间硬球相互作用的数值结果。该理论的定性和定量准确性通过对活性和被动硬磁盘的事件驱动布朗动力学(ED-BD)模拟进行了检验。发现模拟和理论在定量上是一致的,前提是调整整体密度(如从玻璃态动力学的被动描述中所知),并允许在活性主体系统中重新缩放自推进速度。这些调整说明了ABP-MCT通常高估动力学阻滞趋势这一事实。我们在模拟中证实了瞬态和稳态动力学密度相关函数在时间反演下缺乏对称性这一奇特特征,证明了系统的非平衡性质以及它在理论中的表现方式。