Tiliouine I, Delahaye H, Granger G, Leventoux Y, Jimenez C E, Couderc V, Février S
Opt Lett. 2021 Dec 1;46(23):5890-5893. doi: 10.1364/OL.445235.
Fiber-based sources delivering high-energy few-cycle pulses at high repetition rates are currently being developed in the near-infrared spectral range, thanks to the wide availability of telecommunication-grade optical fibers and components. Similar sources in the middle-wave infrared (mid-IR) spectral domain, however, are scarce, although such sources are of high interest for applications such as high-precision frequency metrology and molecular spectroscopy or as a seed source to reach further into the mid-IR via coherent nonlinear processes. Here we report on the design of a fiber-based source of 50-nJ energy 90 fs duration pulses up to 2950 nm, corresponding to 500 kW peak power. To obtain this level of peak power we exploit multi-solitonic fission and soliton self-frequency shift in large mode area fibers excited by picosecond pulses emitted at 2 µm from a megahertz repetition rate fiber laser. We leverage mature silica-based fiber technology up to 2.4 µm and restrict the use of fluoride fiber to the very last frequency-shifting stage. The level of instantaneous power and ultra-short duration achieved in this Letter pave the way to all-fiber format generation of an ultra-broadband coherent continuum in the mid-IR with profound implications for applications such as high-resolution molecular spectroscopy and imaging.
由于电信级光纤和组件的广泛可得性,目前正在近红外光谱范围内开发基于光纤的高重复率高能少周期脉冲源。然而,中波红外(mid-IR)光谱域中的类似光源却很稀少,尽管此类光源对于诸如高精度频率计量和分子光谱学等应用,或者作为通过相干非线性过程进一步深入中红外的种子源而言具有很高的研究价值。在此,我们报告一种基于光纤的光源设计,该光源能产生能量为50 nJ、持续时间为90 fs、波长可达2950 nm的脉冲,对应峰值功率为500 kW。为获得这种峰值功率水平,我们利用了大模面积光纤中的多孤子裂变和孤子自频移,这些光纤由一台兆赫兹重复率光纤激光器在2 µm处发射的皮秒脉冲激发。我们利用成熟的基于二氧化硅的光纤技术,波长可达2.4 µm,并将氟化物光纤的使用限制在最后一个频移阶段。本文所实现的瞬时功率水平和超短持续时间为在中红外波段全光纤形式产生超宽带相干连续谱铺平了道路,这对诸如高分辨率分子光谱学和成像等应用具有深远意义。