Jaksch Sebastian, Pipich Vitaliy, Frielinghaus Henrich
Forschungszentrum Jülich GmbH, Jülich Centre for Neutron Science JCNS-4 at Heinz Maier-Leibnitz Zentrum MLZ, Lichtenbergstrasse 1, D-85747 Garching, Germany.
Technische Universität München TUM, Heinz Maier-Leibnitz Zentrum MLZ, Lichtenbergstrasse 1, D-85747 Garching, Germany.
J Appl Crystallogr. 2021 Oct 20;54(Pt 6):1580-1593. doi: 10.1107/S1600576721009067. eCollection 2021 Dec 1.
This article deals with multiple scattering effects that are important for the method of small-angle neutron scattering (SANS). It considers three channels for the coherent elastic, the incoherent elastic and the incoherent inelastic scattering processes. The first channel contains the desired information on the experiment. Its multiple scattering effects can be desmeared, as shown in the later sections of the article. The other two channels display a nearly constant background as a function of the scattering angle. The incoherent elastic scattering is treated by the theory of Chandrasekhar, allowing for multiple scattering even at large scattering angles. The transfer to a single representative thermalized wavelength by the inelastic scattering - as a simplification - is assumed to happen by a single scattering event. Once the transition to this altered wavelength has happened, further incoherent multiple scattering is considered. The first part of the paper deals with the multiple scattering effects of light water. In the later part of the article, deconvolution algorithms for multiple scattering and instrumental resolution of the elastic coherent signal as implemented in the program are described. All of these considerations are interesting for both reactor-based instruments with velocity selectors and time-of-flight SANS instruments and may improve the reliability of the data treatment.
本文讨论了对小角中子散射(SANS)方法很重要的多重散射效应。它考虑了相干弹性、非相干弹性和非相干非弹性散射过程的三个通道。第一个通道包含实验所需的信息。如本文后面部分所示,其多重散射效应可以被消除。另外两个通道显示出作为散射角函数的几乎恒定的背景。非相干弹性散射由钱德拉塞卡理论处理,即使在大散射角下也允许多重散射。作为一种简化,假设通过单个散射事件发生非弹性散射向单个代表性热化波长的转变。一旦发生向这个改变后的波长的转变,就考虑进一步的非相干多重散射。论文的第一部分讨论了轻水的多重散射效应。在文章的后面部分,描述了程序中实现的用于多重散射的反卷积算法以及弹性相干信号的仪器分辨率。所有这些考虑对于具有速度选择器的基于反应堆的仪器和飞行时间SANS仪器都很有意义,并且可能提高数据处理的可靠性。