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等离子体催化系统中的湿沼气转化

Moist Biogas Conversion in a Plasma-Catalytic System.

作者信息

Młotek Michał, Perron Michalina, Tutaj Katarzyna, Krawczyk Krzysztof

机构信息

Warsaw University of Technology, Noakowskiego 3, 00-664 Warszawa, Poland.

出版信息

ACS Omega. 2021 Dec 6;6(50):34805-34811. doi: 10.1021/acsomega.1c05350. eCollection 2021 Dec 21.

Abstract

The limited resources of conventional fuels and their negative impact on the environment require scientists to search for alternative energy sources. One of the promising renewable sources of energy is biomass. The energy stored in biomass can be used in various ways. It can be combusted, gasified, or fermented, which leads to obtaining biogas. The main components of biogas are carbon dioxide and methane. The aim of this study was to convert in plasma and plasma-catalytic systems low methane biogas into a hydrogen and carbon monoxide mixture, which will allow for a wider range of potential applications. The combustible gas content increased in both systems. The effect of the water vapor content was investigated. It affects the conversion of CH and CO and significantly reduces soot formation (calculated by the carbon balance). It was possible to increase the content of flammable gases by about 20%. The highest molar fraction, 0.16, of hydrogen was obtained with the reduced cobalt catalyst.

摘要

传统燃料资源有限及其对环境的负面影响,要求科学家寻找替代能源。生物质是一种很有前景的可再生能源。生物质中储存的能量可以通过多种方式利用。它可以燃烧、气化或发酵,从而产生沼气。沼气的主要成分是二氧化碳和甲烷。本研究的目的是在等离子体和等离子体催化系统中将低甲烷含量的沼气转化为氢气和一氧化碳的混合物,这将使其具有更广泛的潜在应用范围。在这两种系统中可燃气体含量均有所增加。研究了水蒸气含量的影响。它影响CH和CO的转化,并显著减少烟灰形成(通过碳平衡计算)。可燃气体含量有可能提高约20%。使用还原钴催化剂时获得了最高摩尔分数为0.16的氢气。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4bf2/8697376/79f3f46d4638/ao1c05350_0002.jpg

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