Department of Chemistry - Ångström Laboratory, Uppsala University, 751 21, Uppsala, Sweden.
ABB AB Corporate Research, Forskargränd 7, SE-721 78, Västerås, Sweden.
Chemphyschem. 2022 Apr 5;23(7):e202100829. doi: 10.1002/cphc.202100829. Epub 2022 Mar 1.
The ability to accurately predict lithium-ion battery life-time already at an early stage of battery usage is critical for ensuring safe operation, accelerating technology development, and enabling battery second-life applications. Many models are unable to effectively predict battery life-time at early cycles due to the complex and nonlinear degrading behavior of lithium-ion batteries. In this study, two hybrid data-driven models, incorporating a traditional linear support vector regression (LSVR) and a Gaussian process regression (GPR), were developed to estimate battery life-time at an early stage, before more severe capacity fading, utilizing a data set of 124 battery cells with lifetimes ranging from 150 to 2300 cycles. Two type of hybrid models, here denoted as A and B, were proposed. For each of the models, we achieved 1.1 % (A) and 1.4 % (B) training error, and similarly, 8.3 % (A) and 8.2 % (B) test error. The two key advantages are that the error percentage is kept below 10 % and that very low error values for the training and test sets were observed when utilizing data from only the first 100 cycles.The proposed method thus appears highly promising for predicting battery life during early cycles.
准确预测锂离子电池在使用早期的寿命是确保安全运行、加速技术发展和实现电池二次利用的关键。由于锂离子电池复杂且非线性的退化行为,许多模型无法在早期循环中有效地预测电池寿命。在这项研究中,我们开发了两种混合数据驱动模型,结合了传统的线性支持向量回归(LSVR)和高斯过程回归(GPR),以在早期阶段(在更严重的容量衰减之前)利用一组寿命从 150 到 2300 个循环的 124 个电池的数据集来估计电池寿命。提出了两种类型的混合模型,分别表示为 A 和 B。对于每个模型,我们的训练误差为 1.1%(A)和 1.4%(B),类似地,测试误差为 8.3%(A)和 8.2%(B)。两个关键优势是误差百分比保持在 10%以下,并且当仅使用前 100 个循环的数据时,观察到训练集和测试集的误差值非常低。因此,该方法似乎非常有希望用于预测早期循环中的电池寿命。