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用于稳健飞秒脉冲产生的六方结构硫化镓纳米片的合成

Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation.

作者信息

Guo Kun, Yu Qiang, Liu Fangqi, Deng Haiqin, Yi Tianan, Ren Bo, Su Wei, Zhu Sicong, Wang Zhiqiang, Wu Jian, Zhou Pu

机构信息

College of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, China.

Hubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, The State Key Laboratory for Refractories and Metallurgy, Wuhan University of Science and Technology, Wuhan 430081, China.

出版信息

Nanomaterials (Basel). 2022 Jan 24;12(3):378. doi: 10.3390/nano12030378.

DOI:10.3390/nano12030378
PMID:35159722
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8839219/
Abstract

Gallium sulfide (GaS), with a hexagonal structure, has received extensive attention due to its graphene-like structure and derived optical properties. Here, high-quality GaS was obtained via chemical vapor synthesis and then prepared as a saturable absorber by the stamp-assisted localization-transfer technique onto fiber end face. The stability of the material and the laser damage threshold are maintained due to the optimized thickness and the cavity integration form. The potential of the GaS for nonlinear optics is explored by constructing a GaS-based Erbium-doped mode-locked fiber laser. Stable femtosecond (~448 fs) mode-locking operation of the single pulse train is achieved, and the robust mode-locked operation (>30 days) was recorded. Experimental results show the potential of GaS for multi-functional ultrafast high-power lasers and promote continuous research on graphene-like materials in nonlinear optics and photonics.

摘要

硫化镓(GaS)具有六边形结构,因其类似石墨烯的结构和衍生的光学特性而受到广泛关注。在此,通过化学气相合成获得了高质量的GaS,然后通过印章辅助定位转移技术将其制备成光纤端面上的可饱和吸收体。由于优化的厚度和腔集成形式,材料的稳定性和激光损伤阈值得以保持。通过构建基于GaS的掺铒锁模光纤激光器,探索了GaS在非线性光学方面的潜力。实现了单脉冲序列的稳定飞秒(~448 fs)锁模运行,并记录到了稳健的锁模运行(>30天)。实验结果表明了GaS在多功能超快高功率激光器方面的潜力,并促进了对非线性光学和光子学中类似石墨烯材料的持续研究。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/1a3c9551bbe4/nanomaterials-12-00378-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/136eeeb155dd/nanomaterials-12-00378-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/e39ab4fa79a8/nanomaterials-12-00378-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/5680398b1897/nanomaterials-12-00378-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/02b1b333183f/nanomaterials-12-00378-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/e3364ea370ec/nanomaterials-12-00378-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/1a3c9551bbe4/nanomaterials-12-00378-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/136eeeb155dd/nanomaterials-12-00378-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/e39ab4fa79a8/nanomaterials-12-00378-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/5680398b1897/nanomaterials-12-00378-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/02b1b333183f/nanomaterials-12-00378-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/e3364ea370ec/nanomaterials-12-00378-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0446/8839219/1a3c9551bbe4/nanomaterials-12-00378-g006.jpg

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本文引用的文献

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Front Optoelectron. 2020 Jun;13(2):149-155. doi: 10.1007/s12200-020-1057-4. Epub 2020 Jul 10.
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Femtosecond ultrafast pulse generation with high-quality 2H-TaS nanosheets top-down empirical approach.采用自上而下的经验方法利用高质量2H-TaS纳米片产生飞秒超快脉冲。
Nanoscale. 2021 Dec 16;13(48):20471-20480. doi: 10.1039/d1nr07075d.
3
Two-Dimensional Gallium Sulfide as a Novel Saturable Absorber for Broadband Ultrafast Photonics Applications.
二维硫化镓作为一种用于宽带超快光子学应用的新型可饱和吸收体。
ACS Appl Mater Interfaces. 2021 Dec 29;13(51):61518-61527. doi: 10.1021/acsami.1c18155. Epub 2021 Nov 18.
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PbS Quantum Dots Saturable Absorber for Dual-Wavelength Solitons Generation.用于双波长孤子产生的硫化铅量子点可饱和吸收体
Nanomaterials (Basel). 2021 Sep 29;11(10):2561. doi: 10.3390/nano11102561.
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Study on X-ray Emission Using Ultrashort Pulsed Lasers in Materials Processing.材料加工中使用超短脉冲激光的X射线发射研究。
Materials (Basel). 2021 Aug 12;14(16):4537. doi: 10.3390/ma14164537.
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