Brand Helmut R, Pleiner Harald
Department of Physics, University of Bayreuth, 95440, Bayreuth, Germany.
Max Planck Institute for Polymer Research, 55021, Mainz, Germany.
Eur Phys J E Soft Matter. 2022 Feb 26;45(2):17. doi: 10.1140/epje/s10189-022-00172-8.
We present the macroscopic dynamics of polar nematic liquid crystals in a two-fluid context. We investigate the case of a nonchiral as well as of a chiral solvent. In addition, we analyze how the incorporation of a strain field for polar nematic gels and elastomers in a solvent modifies the macroscopic dynamics. It turns out that the relative velocity between the polar subsystem and the solvent gives rise to a number of cross-coupling terms, reversible as well as irreversible, unknown from the other two-fluid systems considered so far. Possible experiments to study those novel dynamic cross-coupling terms are suggested. As examples we just mention that gradients of the relative velocity lead, in polar nematics to heat currents and in polar cholesterics to temporal changes of the polarization. In polar cholesterics, shear flows give rise to a temporal variation in the velocity difference perpendicular to the shear plane, and in polar nematic gels uniaxial stresses or strains generate temporal variations of the velocity difference.
我们展示了在双流体环境中极性向列相液晶的宏观动力学。我们研究了非手性以及手性溶剂的情况。此外,我们分析了在溶剂中为极性向列相凝胶和弹性体引入应变场如何改变宏观动力学。结果表明,极性子系统与溶剂之间的相对速度产生了许多交叉耦合项,既有可逆的也有不可逆的,这是迄今为止所考虑的其他双流体系统中所没有的。我们提出了研究这些新型动态交叉耦合项的可能实验。例如,我们仅提及相对速度梯度在极性向列相中会导致热流,在极性胆甾相中会导致极化的时间变化。在极性胆甾相中,剪切流会导致垂直于剪切平面的速度差随时间变化,而在极性向列相凝胶中,单轴应力或应变会产生速度差的时间变化。