Ridente Enrico, Mamaikin Mikhail, Altwaijry Najd, Zimin Dmitry, Kling Matthias F, Pervak Vladimir, Weidman Matthew, Krausz Ferenc, Karpowicz Nicholas
Max-Planck-Institut für Quantenoptik, Hans-Kopfermann-Strasse 1, 85748, Garching, Germany.
Fakultät für Physik, Ludwig-Maximilians-Universität, Am Coulombwall 1, 85748, Garching, Germany.
Nat Commun. 2022 Mar 2;13(1):1111. doi: 10.1038/s41467-022-28699-6.
The measurement and control of light field oscillations enable the study of ultrafast phenomena on sub-cycle time scales. Electro-optic sampling (EOS) is a powerful field characterization approach, in terms of both sensitivity and dynamic range, but it has not reached beyond infrared frequencies. Here, we show the synthesis of a sub-cycle infrared-visible pulse and subsequent complete electric field characterization using EOS. The sampled bandwidth spans from 700 nm to 2700 nm (428 to 110 THz). Tailored electric-field waveforms are generated with a two-channel field synthesizer in the infrared-visible range, with a full-width at half-maximum duration as short as 3.8 fs at a central wavelength of 1.7 µm (176 THz). EOS detection of the complete bandwidth of these waveforms extends it into the visible spectral range. To demonstrate the power of our approach, we use the sub-cycle transients to inject carriers in a thin quartz sample for nonlinear photoconductive field sampling with sub-femtosecond resolution.
对光场振荡的测量和控制能够实现亚周期时间尺度上超快现象的研究。电光采样(EOS)就灵敏度和动态范围而言,是一种强大的场表征方法,但它尚未超越红外频率范围。在此,我们展示了亚周期红外 - 可见光脉冲的合成以及随后使用电光采样对完整电场的表征。采样带宽涵盖从700纳米至2700纳米(428至110太赫兹)。通过双信道场合成器在红外 - 可见光范围内生成定制的电场波形,在中心波长1.7微米(176太赫兹)处半高宽持续时间短至3.8飞秒。对这些波形完整带宽的电光采样检测将其扩展到了可见光谱范围。为了展示我们方法的强大之处,我们使用亚周期瞬态在薄石英样品中注入载流子,以实现具有亚飞秒分辨率的非线性光电导场采样。