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粒子数大小分布和新粒子形成于中国东南沿海城市厦门的冬季。

Particle number size distribution and new particle formation in Xiamen, the coastal city of Southeast China in wintertime.

机构信息

CAS Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China; Key Lab of Urban Environment and Health, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China; College of Resources and Environment, Fujian Agriculture and Forest University, Fuzhou 350002, China.

CAS Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China; Key Lab of Urban Environment and Health, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China; College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100086, China.

出版信息

Sci Total Environ. 2022 Jun 20;826:154208. doi: 10.1016/j.scitotenv.2022.154208. Epub 2022 Feb 28.

Abstract

New particle formation (NPF) has a great impact on regional and global climate, air quality and human health. This study uses a Scanning Mobility Particle Sizer (SMPS) for simultaneous measurement of particle number size distribution (PNSD) in wintertime to investigate NPF in the coastal city of Xiamen. The mean particle number concentration, surface area concentration and volume concentration were 7.25 × 10 cm, 152.54 μm cm, and 4.03 μm cm, respectively. Particle number concentration was mainly influenced by the nucleation mode and the Aitken mode, whereas the main contributor to particle surface area concentration and volume concentration was accumulation mode particles. The frequency of NPF events occurred was around 41.4% in December 2019. The typical growth rates of new formed particles were 1.41-2.54 nm h, and the observed formation rates were 0.49-1.43 cm s. A comparative analysis of conditions between event and non-event days was performed. The results emphasized that air temperature, UV radiation and relative humidity were the most decisive meteorological factors, and NPF events usually occurred under clean atmospheric conditions with low PM concentrations. Although condensation sink was high when NPF event occurred, the level of SO and O concentration was also high.

摘要

新粒子形成(NPF)对区域和全球气候、空气质量和人类健康有重大影响。本研究使用扫描迁移率颗粒粒径仪(SMPS)在冬季对粒子数浓度分布(PNSD)进行同步测量,以研究沿海城市厦门的 NPF。平均粒子数浓度、表面积浓度和体积浓度分别为 7.25×10^4cm^-3、152.54μm^2cm^-3和 4.03μm^3cm^-3。粒子数浓度主要受成核模式和艾肯模式的影响,而粒子表面积浓度和体积浓度的主要贡献者是积聚模式粒子。2019 年 12 月 NPF 事件的发生频率约为 41.4%。新形成粒子的典型生长速率为 1.41-2.54nmh^-1,观测到的形成速率为 0.49-1.43cms^-1。对事件日和非事件日的条件进行了对比分析。结果强调,气温、紫外线辐射和相对湿度是最具决定性的气象因素,NPF 事件通常发生在 PM 浓度低、大气清洁的条件下。尽管 NPF 事件发生时凝结阱很高,但 SO 和 O 浓度也很高。

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