Sundaresan Aswathy, Nuchikkat Soniya, Alee K Shadak
School of Physics, IISER - Thiruvananthapuram, Maruthamala PO, Vithura, Thiruvananthapuram, Kerala, 695551, India.
Department of Physics and Nanotechnology, SRM Institute of Science and Technology, Kattankulathur, Chengalpattu (District), Tamil Nadu, 603203, India.
Sci Rep. 2022 Mar 10;12(1):3939. doi: 10.1038/s41598-022-07104-8.
We demonstrate high-quality on chip random lasing of the acceptor dye using a specially designed dynamic linear array of microdroplets with unconventional shapes that do not support the whispering gallery modes. The intrinsic disorder in the droplet array consequent to its dynamic nature is utilized in achieving the randomness in the lasing emission without deliberately adding the disorder as in ordinary random laser systems. The novelty of the generated structure is illustrated by comparing its emission characteristics with two other arrays made of microspheres and microtriangular droplets arranged in a zig zag fashion. We show that only the linear array of microdroplets supports lasing in the acceptor emission. The design of the array structure allows to further reduce the lasing threshold drastically either by incorporating the radiative energy transfer or by tuning the number of acceptor dye molecules. The highly directional, well-controlled, and intense emission of weakly emitting dye generated on chip without the aid of conventional methods opens up a new scheme of random lasing generation mediated by microdroplets.
我们利用一种特殊设计的具有非常规形状的微滴动态线性阵列展示了受体染料的高质量片上随机激光发射,这种微滴形状不支持回音壁模式。由于其动态性质,微滴阵列中固有的无序性被用于实现激光发射的随机性,而不像普通随机激光系统那样刻意添加无序性。通过将其发射特性与另外两种由呈之字形排列的微球和微三角形微滴制成的阵列进行比较,说明了所产生结构的新颖性。我们表明,只有微滴线性阵列支持受体发射中的激光发射。阵列结构的设计允许通过纳入辐射能量转移或调整受体染料分子的数量来进一步大幅降低激光阈值。在没有传统方法辅助的情况下,在芯片上产生的弱发射染料的高度定向、良好控制且强烈的发射开启了一种由微滴介导的随机激光产生的新方案。