Environment Research Institute, Shandong University, Qingdao 266237, China; State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China.
J Environ Sci (China). 2022 Apr;114:170-178. doi: 10.1016/j.jes.2021.08.030. Epub 2021 Aug 23.
To investigate the characteristics of particulate matter with an aerodynamic diameter less than 2.5 μm (PM) and its chemical compositions in the Beijing-Tianjin-Hebei (BTH) region of China during the novel coronavirus disease (COVID-19) lockdown, the ground-based data of PM, trace gases, water-soluble inorganic ions, and organic and elemental carbon were analyzed in three typical cities (Beijing, Tianjin, and Baoding) in the BTH region of China from 5-15 February 2020. The PM source apportionment was established by combining the weather research and forecasting model and comprehensive air quality model with extensions (WRF-CAMx). The results showed that the maximum daily PM concentration reached the heavy pollution level (>150 μg/m) in the above three cities. The sum concentration of SO, NO and NH played a dominant position in PM chemical compositions of Beijing, Tianjin, and Baoding; secondary transformation of gaseous pollutants contributed significantly to PM generation, and the secondary transformation was enhanced as the increased PM concentrations. The results of WRF-CAMx showed obviously inter-transport of PM in the BTH region; the contribution of transportation source decreased significantly than previous reports in Beijing, Tianjin, and Baoding during the COVID-19 lockdown; but the contribution of industrial and residential emission sources increased significantly with the increase of PM concentration, and industry emission sources contributed the most to PM concentrations. Therefore, control policies should be devoted to reducing industrial emissions and regional joint control strategies to mitigate haze pollution.
为了研究新型冠状病毒疾病(COVID-19)封锁期间中国京津冀地区小于 2.5μm 空气动力学直径的颗粒物(PM)及其化学成分的特征,本研究分析了 2020 年 2 月 5 日至 15 日期间中国京津冀地区三个典型城市(北京、天津和保定)的 PM、痕量气体、水溶性无机离子、有机碳和元素碳的地面基础数据。通过结合天气研究和预测模型以及综合空气质量模型与扩展模型(WRF-CAMx),建立了 PM 源分配。结果表明,上述三个城市的 PM 日最大浓度达到重度污染水平(>150μg/m)。SO、NO 和 NH 的总和浓度在北京、天津和保定的 PM 化学成分中占主导地位;气态污染物的二次转化对 PM 的产生有显著贡献,随着 PM 浓度的增加,二次转化增强。WRF-CAMx 的结果表明,京津冀地区的 PM 明显存在相互传输;与之前的报告相比,COVID-19 封锁期间北京、天津和保定的交通源贡献明显下降;但随着 PM 浓度的增加,工业和住宅排放源的贡献显著增加,工业排放源对 PM 浓度的贡献最大。因此,控制政策应致力于减少工业排放,采取区域联合控制策略以减轻雾霾污染。