Institute of Geographic Sciences and Natural Resources Research, CAS, Beijing 100101, China; University of Chinese Academy of Sciences, Beijing 100049, China.
Institute of Geographic Sciences and Natural Resources Research, CAS, Beijing 100101, China; University of Chinese Academy of Sciences, Beijing 100049, China.
Sci Total Environ. 2022 Aug 20;835:155342. doi: 10.1016/j.scitotenv.2022.155342. Epub 2022 Apr 27.
Roadside soils may be affected by potential toxicity elements (TPEs) from vehicles; however, pollution status, ecological and health risks of PTEs in roadside soils were rarely reported on national scale. In this study, a dataset of PTEs in roadside soils was compiled based on the literatures published in 2000-2021, and then pollution level, ecological and health risks of PTEs were evaluated using geochemical accumulation index (I), potential ecological risk index (ER), and human risk assessment coupled with Monte Carlo simulation. Driving factors of PTE accumulation in soils were determined by Geo-detector method. Results indicated that Cd exhibited moderate pollution and considerable ecological risk with the highest I of 1.25 and ER of 100.1, respectively. Vehicle ownership (VP) and precipitation (PP) significantly affected accumulation of PTEs, with q values of 0.209 and 0.191 (P < 0.05), respectively. VP paired with PP enhanced nonlinearly PTE accumulation (q = 0.77). Only 6.89% and 1.54% of non-carcinogenic risks for children and adolescent exceeded the threshold of 1, respectively, whereas 93.11%, 95.67%, 58.80% and 58.14% of carcinogenic risks for senior, adults, adolescent, and children surpassed 1E-06, respectively. The results of this study provided valuable implication for managers to design effective strategies for pollution prevent and risk control.
道路边土壤可能受到车辆潜在毒性元素(TPEs)的影响;然而,道路边土壤中 PTEs 的污染状况、生态和健康风险在国家范围内很少有报道。在本研究中,基于 2000 年至 2021 年发表的文献,编制了道路边土壤中 PTEs 的数据集,然后使用地球化学积累指数(I)、潜在生态风险指数(ER)和人类风险评估与蒙特卡罗模拟相结合的方法来评估 PTEs 的污染水平、生态和健康风险。采用地质探测器方法确定了 PTE 在土壤中积累的驱动因素。结果表明,Cd 表现出中等污染和相当大的生态风险,其 I 值最高为 1.25,ER 值为 100.1。车辆拥有量(VP)和降水量(PP)显著影响 PTE 的积累,q 值分别为 0.209 和 0.191(P<0.05)。VP 与 PP 呈非线性增强 PTE 积累(q=0.77)。只有 6.89%和 1.54%的儿童和青少年非致癌风险超过 1 的阈值,而 93.11%、95.67%、58.80%和 58.14%的老年人、成年人、青少年和儿童致癌风险超过 1E-06。本研究结果为管理者设计有效的污染预防和风险控制策略提供了有价值的启示。