Ranaut Dheeraj, Mukherjee K
School of Basic Sciences, Indian Institute of Technology Mandi, Mandi 175005, Himachal Pradesh, India.
J Phys Condens Matter. 2022 Jun 10;34(31). doi: 10.1088/1361-648X/ac7501.
The realization of an effective spin () ½ state at low temperatures offers a platform to study the enthralling physics behind the disordered states in certain systems. Here, we report the signatures of magnetic ground state associated with= ½ in CeVO. Our studies confirm the absence of any ordering or freezing down to 1.8 K. In the low temperature region, the Curie-Weiss fit of the inverse DC susceptibility indicate towards the presence of antiferromagnetic correlations among the Cespins. The calculated value of effective moment (∼1.16μB) corresponds to= ½ with∼ 1.20. Further, the field dependent magnetization curve at 2 K follows a behaviour corresponding to= ½ Brillouin function with∼ 1.13. Magnetic field dependent heat capacity fits very well with two-level Schottky scheme. Our investigations suggest that CeVOcan be a promising candidate to realise= ½ properties among 3D spin systems.
在低温下实现有效的自旋(1/2)态为研究某些系统中无序态背后引人入胜的物理现象提供了一个平台。在此,我们报告了与CeVO中自旋1/2相关的磁基态特征。我们的研究证实,直至1.8 K都不存在任何有序化或冻结现象。在低温区域,直流磁化率倒数的居里 - 外斯拟合表明Ce自旋之间存在反铁磁关联。有效磁矩的计算值(约1.16μB)对应自旋1/2且朗德因子约为1.20。此外,2 K时的场依赖磁化曲线遵循对应自旋1/2布里渊函数且朗德因子约为1.13的行为。磁场依赖热容量与两能级肖特基模型拟合得非常好。我们的研究表明,CeVO可能是在三维自旋系统中实现自旋1/2特性的一个有前景的候选材料。