School of Optics and Photonics, Beijing Institute of Technology, Beijing 100081, China.
School of Optics and Photonics, Beijing Institute of Technology, Beijing 100081, China.
Spectrochim Acta A Mol Biomol Spectrosc. 2022 Oct 15;279:121418. doi: 10.1016/j.saa.2022.121418. Epub 2022 May 21.
Laser-induced fluorescence (LIF) spectroscopy is widely used for the analysis and classification of olive oil. This paper proposes the classification of LIF data using a specific 1-dimensional convolutional neural network (1D-CNN) model, which does not require pre-processing steps such as normalisation or denoising and can be flexibly applied to massive data. However, by adding a dual convolution structure (Dual-conv) to the model, the features of the 1-dimensional spectra are more scattered within one convolution-pooling process; thus, the classification effects are improved. The models were validated through an olive oil classification experiment which contained a total of 72,000 sets of LIF spectra data, and the classification accuracy rate reached ∼99.69%. Additionally, a common classification approach, the support vector machine (SVM), was utilised for the comparison of the results. The results show that the neural networks perform better than the SVM. The Dual-conv model structure has a faster convergence speed and higher evaluation parameters than those of the 1D-CNN in the same period of iterations, without increasing the data dimension.
激光诱导荧光(LIF)光谱广泛用于橄榄油的分析和分类。本文提出了一种使用特定的一维卷积神经网络(1D-CNN)模型对 LIF 数据进行分类的方法,该模型不需要归一化或去噪等预处理步骤,并且可以灵活应用于海量数据。然而,通过在模型中添加双卷积结构(Dual-conv),可以在一个卷积-池化过程中使一维光谱的特征更加分散,从而提高分类效果。通过一个包含 72000 组 LIF 光谱数据的橄榄油分类实验对模型进行验证,分类准确率达到约 99.69%。此外,还使用支持向量机(SVM)进行了常见的分类方法比较。结果表明,神经网络的性能优于 SVM。在相同的迭代周期内,与 1D-CNN 相比,Dual-conv 模型结构的收敛速度更快,评估参数更高,而不会增加数据维度。