Department of Chemistry and Stanford ChEM-H, Stanford University, Stanford, 94305, CA, USA.
Department of Chemistry, Yale University, New Haven, 06511, CT, USA.
Nat Commun. 2022 Jun 20;13(1):3542. doi: 10.1038/s41467-022-31062-4.
Mucin domains are densely O-glycosylated modular protein domains found in various extracellular and transmembrane proteins. Mucin-domain glycoproteins play important roles in many human diseases, such as cancer and cystic fibrosis, but the scope of the mucinome remains poorly defined. Recently, we characterized a bacterial O-glycoprotease, StcE, and demonstrated that an inactive point mutant retains binding selectivity for mucin-domain glycoproteins. In this work, we leverage inactive StcE to selectively enrich and identify mucin-domain glycoproteins from complex samples like cell lysate and crude ovarian cancer patient ascites fluid. Our enrichment strategy is further aided by an algorithm to assign confidence to mucin-domain glycoprotein identifications. This mucinomics platform facilitates detection of hundreds of glycopeptides from mucin domains and highly overlapping populations of mucin-domain glycoproteins from ovarian cancer patients. Ultimately, we demonstrate our mucinomics approach can reveal key molecular signatures of cancer from in vitro and ex vivo sources.
粘蛋白结构域是富含 O-糖基化的模块化蛋白结构域,存在于各种细胞外和跨膜蛋白中。粘蛋白结构域糖蛋白在许多人类疾病中发挥着重要作用,如癌症和囊性纤维化,但粘蛋白组的范围仍未得到明确界定。最近,我们鉴定了一种细菌 O-糖基化酶 StcE,并证实一种无活性的点突变体仍保留对粘蛋白结构域糖蛋白的结合选择性。在这项工作中,我们利用无活性的 StcE 从细胞裂解物和粗卵巢癌患者腹水等复杂样本中选择性地富集和鉴定粘蛋白结构域糖蛋白。我们的富集策略还得到了一种算法的辅助,该算法可以为粘蛋白结构域糖蛋白鉴定分配置信度。该粘蛋白组学平台可以从卵巢癌患者中检测到数百个来自粘蛋白结构域的糖肽和高度重叠的粘蛋白结构域糖蛋白群体。最终,我们证明我们的粘蛋白组学方法可以从体外和体内来源揭示癌症的关键分子特征。