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石墨烯纳米带中强大的自旋相关塞贝克效应及卓越的自旋热电性能。

A robust spin-dependent Seebeck effect and remarkable spin thermoelectric performance in graphether nanoribbons.

作者信息

Jiang Yue, Guo Yan-Dong, Lin Li-Yan, Yan Xiao-Hong

机构信息

College of Electronic and Optical Engineering, Nanjing University of Posts and Telecommunications, Nanjing 210046, China.

College of Science, Jinling Institute of Technology, Nanjing 211169, China.

出版信息

Nanoscale. 2022 Jul 21;14(28):10033-10040. doi: 10.1039/d2nr02175g.

Abstract

The generation of spin currents is a significant issue in spintronics. A spin current can be induced by a temperature gradient in the spin-dependent Seebeck effect, which has attracted growing interest over recent years. Herein we propose spin caloritronic devices based on magnetic graphether nanoribbons and investigate the spin thermoelectric properties by first-principles calculations. Owing to the symmetrical spin-resolved transmission spectra, our devices exhibit a robust spin-dependent Seebeck effect and could generate a pure spin current. Moreover, they manifest a high spin Seebeck coefficient and a giant spin figure of merit. Our findings demonstrate that graphether-nanoribbon-based devices possess remarkable spin thermoelectric performance, and might be promising candidates for spin caloritronics.

摘要

自旋电流的产生是自旋电子学中的一个重要问题。在自旋相关的塞贝克效应中,温度梯度可以诱导产生自旋电流,近年来这一效应已引起越来越多的关注。在此,我们提出了基于磁性石墨烯纳米带的自旋热电器件,并通过第一性原理计算研究其自旋热电性质。由于自旋分辨传输谱的对称性,我们的器件表现出稳健的自旋相关塞贝克效应,并且能够产生纯自旋电流。此外,它们还表现出高自旋塞贝克系数和巨大的自旋优值。我们的研究结果表明,基于石墨烯纳米带的器件具有卓越的自旋热电性能,可能是自旋热电子学的有前途的候选者。

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