Three-dimensional nature of summertime aerosols over South Asia.

Three-dimensional (temporal-spatial-vertical) climatology of South Asian summertime (MAMJ, 2010-2019) aerosols and aerosol sub-types was explored using multiple high-resolution satellite-based observations and reanalysis dataset. Vertical stratification of aerosol layer and aerosol sub-types was identified using observation from space-borne lidar. Aerosol optical depth (AOD) was particularly high across the Indo-Gangetic Plain (IGP; AOD ± SD: 0.56 ± 0.12) and over eastern coast of India (AOD: 0.6-0.8), with prevalence of heterogeneous aerosol sub-types having strong spatial gradient. Clearly, aerosols over north-western arid part were highly absorbing (Ultra-violet Aerosol Index, UVAI > 0.80) and coarse (Ångström exponent, AE < 0.8), with an indication of desert/-mineral dust aerosols. In contrast, fine and moderate to non-absorbing aerosols (UVAI: 0.20-0.50) dominate from central to lower IGP, including in Bangladesh, with signature of anthropogenic emissions. Prevailing aerosols over twelve South Asian cities were classified into six aerosol sub-types constraining their particle size and UV-absorbing potential. Overall, mineral dust, smoke and urban aerosols were the three major aerosol sub-types that prevail across South Asia during summer. In particular, 58-70 % of retrieval days over Karachi and Multan were dust dominated; 57-64 % days were dust or urban aerosols dominated over Lahore, Delhi, Kanpur and Varanasi, and 56-77 % days were smoke or urban aerosols dominated over Dhaka, Kathmandu, Chennai, Mumbai, Colombo and Nagpur. Prevailing aerosols were vertically stratified as 50-70 % of total AOD was retrieved <2 km from the surface except in few cities where 70-80 % of AOD was retrieved <3 km height. Mineral dust and/or urban aerosols emerged as the most abundant aerosol types near the surface (<1 km) in all the cities except in Chennai, with their abundance remained as a function of emission sources and geographical location.