Geological Oceanography Division, CSIR-National Institute of Oceanography, Dona Paula, India.
Geosciences Division, Physical Research Laboratory, Ahmedabad, India.
J Air Waste Manag Assoc. 2022 Oct;72(10):1161-1173. doi: 10.1080/10962247.2022.2100509. Epub 2022 Sep 8.
Atmospheric aerosol over the Arabian Sea is significantly impacted by the long-range transported mineral dust from the surrounding continents. This transported mineral dust is hypothesized and tested during several studies to see the impacts on the surface ocean biogeochemical processes and subsequently to the Carbon cycle. It is, thus important to quantify dust contributions and their fluxes to the Arabian Sea. Here we assess temporal variability of dust concentration, their elemental characteristics as well as quantify their dry and wet deposition fluxes over the North-eastern Arabian Sea. The dust concentrations were found to vary from 59 to 132 µg m which accounts for 50% to 90% of total mass during dusty days. However, its contribution during pre and post dust storms ranges between 6% and 60%. Relatively higher dust dry deposition flux of 28 ± 7 mg m day (range: 20-44) is estimated for dusty days compared to pre and post dusty days (range: 0.4-22 mg m day). In contrast to dry deposition fluxes, significantly higher fluxes are estimated from wet deposition, averaging around 240 ± 220 mg m day. These values are five times higher than those reported from cruise samples collected over the Arabian Sea. The contribution of dust to aerosol mass is further ascertained using elemental composition, wherein a significant correlation was observed between Fe and Al (r = 0.77) for samples collected during the dusty period, highlighting their similar crustal sources. Our estimation of dust flux over this region has implications for the supply of nutrients associated with natural dust to the surface water of the Arabian Sea. The Arabian Sea, one of the productive oceanic regions among the global oceans, has been identified as a perennial source of atmospheric CO. This basin is heavily impacted by atmospheric dust deposition/inputs owing to its geographical location being surrounded by arid and semi-arid regions. It has been hypothesized that aeolian dust plays a significant role in modulating surface water biogeochemical processes including primary productivity, in the Arabian Sea. Furthermore, modelling studies have highlighted on the role of dust (containing Fe) in fueling and enhancing primary productivity in the Arabian Sea. However, quantification of dust deposition fluxes (wet and dry) on seasonal time scale is missing in the literature. This paper aims to partially fulfil this research gap by providing a long-term data of wet and dry deposition fluxes over the northeastern Arabian Sea. We have also discussed their seasonal variability and factors affecting this flux. Thus, this study will be valuable contribution to the aeolian research community and have significant implication toward the role of aeolian deposition to the surface water biogeochemical processes in the Arabian Sea.
阿拉伯海上空的大气气溶胶受到来自周边大陆的长距离传输矿物粉尘的显著影响。在几项研究中,人们假设并测试了这种传输矿物粉尘对表层海洋生物地球化学过程的影响,进而对碳循环产生影响。因此,量化粉尘的贡献及其向阿拉伯海的通量是很重要的。在这里,我们评估了东北阿拉伯海上的粉尘浓度、元素特征及其干湿沉降通量的时间变化。研究发现,在多尘日,粉尘浓度从 59 到 132µg m 变化,占总质量的 50%到 90%。然而,在沙尘前后,其贡献范围在 6%到 60%之间。与沙尘前后相比,在多尘日,相对较高的粉尘干沉降通量为 28±7mg m 天(范围:20-44)。与干沉降通量相反,从湿沉降中估计的通量要高得多,平均约为 240±220mg m 天。这些值是从阿拉伯海上收集的巡航样本报告值的五倍。通过元素组成进一步确定了粉尘对气溶胶质量的贡献,其中在多尘期间收集的样品中观察到 Fe 和 Al 之间存在显著相关性(r=0.77),突出了它们的相似地壳来源。我们对该地区粉尘通量的估计对与天然粉尘相关的营养物质向阿拉伯海表层水的供应具有重要意义。阿拉伯海是全球海洋中生产力较高的海洋区域之一,被认为是大气 CO 的常年来源。由于其地理位置被干旱和半干旱地区环绕,这个盆地受到大气粉尘沉积/输入的严重影响。人们假设,风尘在调节阿拉伯海的表层水生物地球化学过程(包括初级生产力)方面发挥了重要作用。此外,建模研究强调了粉尘(含有 Fe)在阿拉伯海激发和增强初级生产力方面的作用。然而,文献中缺少季节性时间尺度上的粉尘沉降通量(干湿)的定量数据。本文旨在通过提供东北阿拉伯海上的干湿沉降通量的长期数据来部分填补这一研究空白。我们还讨论了它们的季节性变化和影响这种通量的因素。因此,这项研究将是对风尘研究界的一个有价值的贡献,并对风尘对阿拉伯海表层水生物地球化学过程的作用具有重要意义。