Guangdong Provincial Key Laboratory of Water and Air Pollution Control, South China Institute of Environmental Science, Ministry of Ecology and Environment, Guangzhou 510655, China; School of Environment and Energy, South China University of Technology, Guangzhou 510006, China.
Guangdong Provincial Key Laboratory of Water and Air Pollution Control, South China Institute of Environmental Science, Ministry of Ecology and Environment, Guangzhou 510655, China.
Sci Total Environ. 2022 Nov 10;846:157317. doi: 10.1016/j.scitotenv.2022.157317. Epub 2022 Jul 13.
Cooking in China supply the large population with nutrition and, as a commercial activity, it also promotes the economic growth of Chinese society. The specific cooking styles in China can produce complex volatile organic compound (VOC) emissions. The resulting adverse effects on the environment and human health of carbonyls from cooking should not be ignored. We quantitatively evaluated the contribution of carbonyls to common VOCs (carbonyl/VOC ratio) from cooking activities in China through the establishment and comparison of the source profiles, emission factors (EFs), emission amount and ozone formation potential (OFP). It was found that carbonyls are crucial components of VOCs from commercial, canteen and residential cooking activities (COC, CAC and REC, respectively). The carbonyl/VOC ratio from cooking activities in China had EFs, emissions, and a total OFP of 22-65 %, 23-34 %, and 49-104 %, respectively. The high OFP was due to the high OFP emissions intensity (OFP) and maximum incremental reactivity (MIR) values of carbonyls. This indicates that to alleviate O pollution, OFP-based control measures that target carbonyls might be more efficient than measures that target common VOCs. Priority should be given to emission controlling COC emissions, specifically those from medium- and large-scale catering. Formaldehyde, acetaldehyde, and hexanal were the key carbonyl species that form O in the environment. Our findings imply that cooking-emitted carbonyls should not be overlooked in investigations of O formation and that these compounds should be subject to strict regulations.
在中国,烹饪不仅为庞大的人口提供了营养,而且作为一种商业活动,也促进了中国社会的经济增长。中国特有的烹饪风格会产生复杂的挥发性有机化合物(VOC)排放。烹饪过程中羰基化合物对环境和人体健康产生的不利影响不容忽视。我们通过建立和比较源谱、排放因子(EF)、排放量和臭氧形成潜力(OFP),定量评估了烹饪活动中羰基化合物对常见 VOCs(羰基/VOC 比)的贡献。结果表明,羰基化合物是商业烹饪、食堂烹饪和居民烹饪活动(COC、CAC 和 REC)中 VOC 的重要组成部分。中国烹饪活动的羰基/VOC 比的 EF、排放和总 OFP 分别为 22-65%、23-34%和 49-104%。高 OFP 是由于羰基化合物的高 OFP 排放强度(OFP)和最大增量反应性(MIR)值。这表明,为了缓解 O 污染,基于 OFP 的控制措施针对羰基化合物可能比针对常见 VOCs 的措施更有效。应优先控制 COC 排放,特别是中型和大型餐饮的排放。甲醛、乙醛和己醛是环境中形成 O 的关键羰基物质。我们的研究结果表明,在研究 O 形成时不应忽视烹饪排放的羰基化合物,这些化合物应受到严格监管。