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巴基斯坦克乌拉盐矿的热释光 NaCl 颗粒的剂量学特性。

Dosimetric properties of thermoluminescent NaCl pellets from Khewra Salt Mines, Pakistan.

机构信息

Department of Physics & Applied Mathematics, Pakistan Institute of Engineering and Applied Sciences (PIEAS), Islamabad, Pakistan.

Health Physics Division, Pakistan Institute of Nuclear Sciences and Technology (PINSTECH), Islamabad, Pakistan.

出版信息

Luminescence. 2022 Oct;37(10):1701-1709. doi: 10.1002/bio.4345. Epub 2022 Aug 3.

DOI:10.1002/bio.4345
PMID:35864081
Abstract

Thermoluminescence (TL) and extended dosimetric characteristics of naturally occurring sodium chloride (NaCl) salt were studied. Pellets were prepared from mined crystalline salt obtained from Khewra Salt Mines, Pakistan and irradiated from 1 mGy to 10,000 mGy using cobalt-60 gamma source. The TL response showed two dominant peaks around 125°C and 230°C, respectively, at low doses, with an additional peak in between at doses beyond 300 mGy. A linear and supra-linear TL response was observed between 1 mGy-100 mGy and 100 mGy-10 Gy dose ranges, respectively. During the first 24 h post-irradiation, the TL intensity dropped by 20%. A maximum angular dependence of up to 50% was observed between 0° to 360°. For photon energies between 33 keV and 1.25 MeV significant energy dependence was observed for photons < 100 keV only. Sample sensitivity increased with dose a qualitatively similar behaviour to TLD-200. Effective atomic number (Z ) of the sample (14.6) was comparable to TLD-200 (16.3). No significant dose rate effects (deviation for a cobalt-60 source within 3.5%) on the TL sensitivity of the sample were found. The lowest detectable dose limit (LDDL) for salt sample was found to be 0.8 mGy whereas the sample reproducibility test showed a maximum of ±11% deviation from the first value.

摘要

研究了天然氯化钠 (NaCl) 盐的热释光 (TL) 和扩展剂量特性。从巴基斯坦克乌拉盐矿开采的结晶盐制成了颗粒,并使用钴-60 伽马源从 1 mGy 照射到 10000 mGy。TL 响应在低剂量下分别在 125°C 和 230°C 左右显示出两个主要峰值,在超过 300 mGy 的剂量之间还有一个额外的峰值。在 1 mGy-100 mGy 和 100 mGy-10 Gy 剂量范围内分别观察到线性和超线性 TL 响应。在辐照后 24 小时内,TL 强度下降了 20%。在 0°至 360°之间观察到最大角度依赖性高达 50%。对于光子能量在 33 keV 和 1.25 MeV 之间,仅在光子能量 < 100 keV 时观察到明显的能量依赖性。样品灵敏度随剂量增加而增加,与 TLD-200 的行为相似。样品的有效原子数 (Z)(14.6)与 TLD-200(16.3)相当。未发现样品 TL 灵敏度的显著剂量率效应(钴-60 源内偏差 3.5%)。盐样品的最低可检测剂量限值 (LDDL) 发现为 0.8 mGy,而样品重复性测试显示从第一个值最大偏差为±11%。

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