Leung Casey K W, Zhang Xiaofu, von Rohr Fabian, Lortz Rolf, Jäck Berthold
Department of Physics, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong SAR, China.
State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences (CAS), Shanghai, 200050, China.
Sci Rep. 2022 Jul 27;12(1):12773. doi: 10.1038/s41598-022-16355-4.
High-entropy alloys (HEA) form through the random arrangement of five or more chemical elements on a crystalline lattice. Despite the significant amount of resulting compositional disorder, a subset of HEAs enters a superconducting state below critical temperatures, [Formula: see text] K. The superconducting properties of the known HEAs seem to suffice a Bardeen-Cooper-Schrieffer (BCS) description, but little is known about their superconducting order parameter and the microscopic role of disorder. We report on magnetic susceptibility measurements on films of the superconducting HEA (TaNb)Formula: see text[Formula: see text] for characterizing the lower and upper critical fields [Formula: see text] and [Formula: see text], respectively as a function of temperature T. Our resulting analysis of the Ginzburg-Landau coherence length and penetration depth demonstrates that HEAs of this type are single-band isotropic s-wave superconductors in the dirty limit. Despite a significant difference in the elemental composition between the [Formula: see text] and [Formula: see text] films, we find that the observed [Formula: see text] variations cannot be explained by disorder effects.
高熵合金(HEA)是通过五种或更多化学元素在晶格上的随机排列形成的。尽管由此产生了大量的成分无序,但一部分高熵合金在低于临界温度((T_c)),即(T_c < 2) K时进入超导状态。已知高熵合金的超导特性似乎符合巴丁 - 库珀 - 施里弗(BCS)描述,但对其超导序参量以及无序的微观作用了解甚少。我们报告了对超导高熵合金(TaNb)({0.5})(ZrHfTi)({0.5})薄膜的磁化率测量结果,以分别表征作为温度(T)函数的下临界场(H_{c1})和上临界场(H_{c2})。我们对金兹堡 - 朗道相干长度和穿透深度的分析结果表明,这种类型的高熵合金在脏极限下是单带各向同性的(s)波超导体。尽管(TaNb)({0.5})(ZrHfTi)({0.5})薄膜与(TaNb)({0.6})(ZrHfTi)({0.4})薄膜之间的元素组成存在显著差异,但我们发现观察到的(H_{c2})变化无法用无序效应来解释。